ArticlePolymer science. Series A, Chemistry, physics2016
Electrostatic Correlations in Polyelectrolyte Solutions.
Article in Polymer science. Series A, Chemistry, physics, 2016. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Extreme dependence of dynamics on concentration in highly crowded polyelectrolyte solutions.Science advances · 2024Article
- Tuning Net Charge in Aliphatic Polycarbonates Alters Solubility and Protein Complexation Behavior.ACS omega · 2021Article
- Theory of Charged Gels: Swelling, Elasticity, and Dynamics.Gels (Basel, Switzerland) · 2021Review
- Article
- Disappearance of the polyelectrolyte peak in salt-free solutions.Physical review. E · 2020Article
- A unified analytical theory of heteropolymers for sequence-specific phase behaviors of polyelectrolytes and polyampholytes.The Journal of chemical physics · 2020Article
- Polyelectrolyte association and solvation.The Journal of chemical physics · 2018Article
- Communication: Counter-ion solvation and anomalous low-angle scattering in salt-free polyelectrolyte solutions.The Journal of chemical physics · 2017Article
- Review
Corrections and comments
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Authors and funding
1 author.
Funding
Abstract
The major attribute of polyelectrolyte solutions is that all chains are strongly correlated both electrostatically and topologically. Even in very dilute solutions such that the chains are not interpenetrating, the chains are still strongly correlated. These correlations are manifest in the measured scattering intensity when such solutions are subjected to light, X-ray, and neutron radiation. The behavior of scattering intensity from polyelectrolyte solutions is qualitatively different from that of solutions of uncharged polymers. Using the technique introduced by Sir Sam Edwards, and extending the earlier work by the author on the thermodynamics of polyelectrolyte solutions, extrapolation formulas are derived for the scattering intensity from polyelectrolyte solutions. The emergence of the polyelectrolyte peak and its concentration dependence are derived. The derived theory shows that there are five regimes. Published experimental data from many laboratories are also collected into a master figure and a comparison between the present theory and experiments is presented.
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Registered trials
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