ArticleProceedings of the National Academy of Sciences of the United States of America2018
Water-like anomalies as a function of tetrahedrality.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 20 papers.
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Who cites it
20 citing papers in PubMed.
- The Rose Model of Water: Linking Theory and Simulation.Entropy (Basel, Switzerland) · 2026Article
- Assessing Order in Liquid, Supercooled, and Crystalline Water.The journal of physical chemistry. B · 2026Article
- From Upconversion Nanoparticles to Proteins: Probing Hydration-Water Density Fluctuations by Luminescence Thermometry.Accounts of chemical research · 2026Article
- Competing hydrogen-bond orders drive water's anomalous surface tension.Nature communications · 2026Article
- Protein Confinement Decouples Dynamical Heterogeneity from Structural Preordering in Supercooled Monolayer Water.JACS Au · 2025Article
- Anomalous Water Fluorescence Induced by Solutes.The journal of physical chemistry letters · 2025Article
- Snowflake Model of Water: A Fast Approach for Calculation of Structural Properties of Liquid Water.Journal of chemical theory and computation · 2025Article
- Structural Origin of Dynamic Heterogeneity in Supercooled Liquids.The journal of physical chemistry. B · 2025Review
- Dynamic anti-correlations of water hydrogen bonds.Nature communications · 2024Article
- Evidence of ferroelectric features in low-density supercooled water from ab initio deep neural-network simulations.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- Deciphering Density Fluctuations in the Hydration Water of Brownian Nanoparticles via Upconversion Thermometry.The journal of physical chemistry letters · 2024Article
- Are Neural Network Potentials Trained on Liquid States Transferable to Crystal Nucleation? A Test on Ice Nucleation in the mW Water Model.The journal of physical chemistry. B · 2023Article
- Two-dimensional infrared-Raman spectroscopy as a probe of water's tetrahedrality.Nature communications · 2023Article
- Advances in the study of supercooled water.The European physical journal. E, Soft matter · 2021Review
- Statistical Mechanics and Thermodynamics of Liquids and Crystals.Entropy (Basel, Switzerland) · 2021Article
- A hierarchical clustering method of hydrogen bond networks in liquid water undergoing shear flow.Scientific reports · 2021Article
- The anomalies and criticality of liquid water.Proceedings of the National Academy of Sciences of the United States of America · 2020Article
- Signatures of a liquid-liquid transition in an ab initio deep neural network model for water.Proceedings of the National Academy of Sciences of the United States of America · 2020Article
- A new topological descriptor for water network structure.Journal of cheminformatics · 2019Article
- Ice is born in low-mobility regions of supercooled liquid water.Proceedings of the National Academy of Sciences of the United States of America · 2019Article
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Authors and funding
3 authors.
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Abstract
Tetrahedral interactions describe the behavior of the most abundant and technologically important materials on Earth, such as water, silicon, carbon, germanium, and countless others. Despite their differences, these materials share unique common physical behaviors, such as liquid anomalies, open crystalline structures, and extremely poor glass-forming ability at ambient pressure. To reveal the physical origin of these anomalies and their link to the shape of the phase diagram, we systematically study the properties of the Stillinger-Weber potential as a function of the strength of the tetrahedral interaction [Formula: see text] We uncover a unique transition to a reentrant spinodal line at low values of [Formula: see text], accompanied with a change in the dynamical behavior, from non-Arrhenius to Arrhenius. We then show that a two-state model can provide a comprehensive understanding on how the thermodynamic and dynamic anomalies of this important class of materials depend on the strength of the tetrahedral interaction. Our work establishes a deep link between the shape of the phase diagram and the thermodynamic and dynamic properties through local structural ordering in liquids and hints at why water is so special among all substances.
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