ArticleNature communications2018
Three-dimensional localization of nanoscale battery reactions using soft X-ray tomography.
Article in Nature communications, 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 22 papers.
What it found
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Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
22 citing papers in PubMed.
- Three-dimensional imaging of sulfur chemical states in polymers with micrometer thickness using sulfur K-edge ptychographic tomography.Scientific reports · 2026Article
- Revealing the degradation pathways of layered Li-rich oxide cathodes.Nature nanotechnology · 2024Article
- Rational partitioning of spectral feature space for effective clustering of massive spectral image data.Scientific reports · 2024Article
- Optimal Sparse Energy Sampling for X-ray Spectro-Microscopy: Reducing the X-ray Dose and Experiment Time Using Model Order Reduction.Chemical & biomedical imaging · 2024Article
- Soft X-ray spectro-ptychography of boron nitride nanobamboos, carbon nanotubes and permalloy nanorods.Journal of synchrotron radiation · 2023Article
- Understanding the microstructure of a core-shell anode catalyst layer for polymer electrolyte water electrolysis.Scientific reports · 2023Article
- Differential phase contrast for quantitative imaging and spectro-microscopy at a nanoprobe beamline.Journal of synchrotron radiation · 2023Article
- Artificial Intelligence Applied to Battery Research: Hype or Reality?Chemical reviews · 2022Review
- Bridging nano- and microscale X-ray tomography for battery research by leveraging artificial intelligence.Nature nanotechnology · 2022Review
- X-ray Spectroptychography.ACS omega · 2022Review
- Effect of crystallite geometries on electrochemical performance of porous intercalation electrodes by multiscale operando investigation.Nature materials · 2022Article
- Article
- Sparse ab initio x-ray transmission spectrotomography for nanoscopic compositional analysis of functional materials.Science advances · 2021Article
- The Hard X-ray Nanoprobe beamline at Diamond Light Source.Journal of synchrotron radiation · 2021Article
- Upscaling X-ray nanoimaging to macroscopic specimens.Journal of applied crystallography · 2021Review
- Local Substrate Heterogeneity Influences Electrochemical Activity of TEM Grid-Supported Battery Particles.Frontiers in chemistry · 2021Article
- Depth-dependent valence stratification driven by oxygen redox in lithium-rich layered oxide.Nature communications · 2020Article
- An ultrahigh-resolution soft x-ray microscope for quantitative analysis of chemically heterogeneous nanomaterials.Science advances · 2020Article
- Iterative X-ray spectroscopic ptychography.Journal of applied crystallography · 2020Article
- Machine-learning-revealed statistics of the particle-carbon/binder detachment in lithium-ion battery cathodes.Nature communications · 2020Article
Corrections and comments
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Authors and funding
19 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Battery function is determined by the efficiency and reversibility of the electrochemical phase transformations at solid electrodes. The microscopic tools available to study the chemical states of matter with the required spatial resolution and chemical specificity are intrinsically limited when studying complex architectures by their reliance on two-dimensional projections of thick material. Here, we report the development of soft X-ray ptychographic tomography, which resolves chemical states in three dimensions at 11 nm spatial resolution. We study an ensemble of nano-plates of lithium iron phosphate extracted from a battery electrode at 50% state of charge. Using a set of nanoscale tomograms, we quantify the electrochemical state and resolve phase boundaries throughout the volume of individual nanoparticles. These observations reveal multiple reaction points, intra-particle heterogeneity, and size effects that highlight the importance of multi-dimensional analytical tools in providing novel insight to the design of the next generation of high-performance devices.
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Registered trials
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