ArticleThe journal of physical chemistry. B2018
Structure from Dynamics: Vibrational Dynamics of Interfacial Water as a Probe of Aqueous Heterogeneity.
Article in The journal of physical chemistry. B, 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 15 papers.
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Who cites it
15 citing papers in PubMed.
- Mimicking on-water surface synthesis through micellar interfaces.Nature communications · 2024Article
- How Thick is the Air-Water Interface?─A Direct Experimental Measurement of the Decay Length of the Interfacial Structural Anisotropy.Langmuir : the ACS journal of surfaces and colloids · 2024Article
- Molecular dynamics simulation study of water structure and dynamics on the gold electrode surface with adsorbed 4-mercaptobenzonitrile.The Journal of chemical physics · 2024Article
- The hydrogen-bonding dynamics of water to a nitrile-functionalized electrode is modulated by voltage according to ultrafast 2D IR spectroscopy.Proceedings of the National Academy of Sciences of the United States of America · 2023Article
- Electrostatic switch mechanisms of membrane protein trafficking and regulation.Biophysical reviews · 2023Review
- Water at charged interfaces.Nature reviews. Chemistry · 2021Review
- Hydrogen bond dynamics of interfacial water molecules revealed from two-dimensional vibrational sum-frequency generation spectroscopy.Scientific reports · 2021Article
- Mapping the temperature-dependent and network site-specific onset of spectral diffusion at the surface of a water cluster cage.Proceedings of the National Academy of Sciences of the United States of America · 2020Article
- Spatially dependent H-bond dynamics at interfaces of water/biomimetic self-assembled lattice materials.Proceedings of the National Academy of Sciences of the United States of America · 2020Article
- Vibrational Spectroscopic Map, Vibrational Spectroscopy, and Intermolecular Interaction.Chemical reviews · 2020Review
- Interfacial Vibrational Dynamics of Ice IJournal of the American Chemical Society · 2020Article
- Molecular Structure and Modeling of Water-Air and Ice-Air Interfaces Monitored by Sum-Frequency Generation.Chemical reviews · 2020Article
- Unveiling Heterogeneity of Interfacial Water through the Water Bending Mode.The journal of physical chemistry letters · 2019Article
- Phase-Sensitive Sum-Frequency Generation Measurements Using a Femtosecond Nonlinear Interferometer.The journal of physical chemistry. C, Nanomaterials and interfaces · 2019Article
- Polar Interactions Play an Important Role in the Energetics of the Main Phase Transition of Phosphatidylcholine Membranes.ACS omega · 2019Article
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Authors and funding
4 authors.
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Abstract
The structural heterogeneity of water at various interfaces can be revealed by time-resolved sum-frequency generation spectroscopy. The vibrational dynamics of the O-H stretch vibration of interfacial water can reflect structural variations. Specifically, the vibrational lifetime is typically found to increase with increasing frequency of the O-H stretch vibration, which can report on the hydrogen-bonding heterogeneity of water. We compare and contrast vibrational dynamics of water in contact with various surfaces, including vapor, biomolecules, and solid interfaces. The results reveal that variations in the vibrational lifetime with vibrational frequency are very typical, and can frequently be accounted for by the bulk-like heterogeneous response of interfacial water. Specific interfaces exist, however, for which the behavior is less straightforward. These insights into the heterogeneity of interfacial water thus obtained contribute to a better understanding of complex phenomena taking place at aqueous interfaces, such as photocatalytic reactions and protein folding.
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