Evidence map›Paper›PMID 29372181›Full record

ArticleScience advances2018

Dynamic traction of lattice-confined platinum atoms into mesoporous carbon matrix for hydrogen evolution reaction.

Huabin Zhang, Pengfei An, Wei Zhou, Bu Yuan Guan, Peng Zhang, Juncai Dong, Xiong Wen David Lou

Open access · goldAbstract read
In one paragraph

Article in Science advances, 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 57 papers.

0numbers the graph read from it
0cells of the map it votes in
57citing papers in PubMed
19.6field-weighted citation impact, top 1% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

57 citing papers in PubMed, 575 citations in OpenAlex.

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  15. Steering lithium and potassium storage mechanism in covalent organic frameworks by incorporating transition metal single atoms.Proceedings of the National Academy of Sciences of the United States of America · 2024
    Article
  16. A universal and scalable transformation of bulk metals into single-atom catalysts in ionic liquids.Proceedings of the National Academy of Sciences of the United States of America · 2024
    Article
  17. Article
  18. Boosted hydrogen evolution kinetics of heteroatom-doped carbons with isolated Zn as an accelerant.Proceedings of the National Academy of Sciences of the United States of America · 2024
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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

7 authors at 3 institutions in 3 countries.

Huabin ZhangSchool of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive, Singapore 637459, Singapore.ORCID 0000-0003-1601-2471
Pengfei AnBeijing Synchrotron Radiation Facility, Institute of High Energy Physics, Chinese Academy of Sciences, Beijing 100049, China.ORCID 0000-0001-7231-4218
Wei ZhouDepartment of Applied Physics, Tianjin Key Laboratory of Low Dimensional Materials Physics and Preparing Technology, Faculty of Science, Tianjin University, Tianjin 300072, P. R. China.ORCID 0000-0002-8004-3996
Bu Yuan GuanSchool of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive, Singapore 637459, Singapore.
Peng ZhangSchool of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive, Singapore 637459, Singapore.ORCID 0000-0003-2228-3569
Juncai DongBeijing Synchrotron Radiation Facility, Institute of High Energy Physics, Chinese Academy of Sciences, Beijing 100049, China.ORCID 0000-0001-8860-093X
Xiong Wen David LouSchool of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive, Singapore 637459, Singapore.ORCID 0000-0002-5557-4437
Nanyang Technological University · SGChinese Academy of Sciences · CNTianjin University · CN

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Constructing atomically dispersed platinum (Pt) electrocatalysts is essential to build high-performance and cost-effective electrochemical water-splitting systems. We present a novel strategy to realize the traction and stabilization of isolated Pt atoms in the nitrogen-containing porous carbon matrix (Pt@PCM). In comparison with the commercial Pt/C catalyst (20 weight %), the as-prepared Pt@PCM catalyst exhibits significantly boosted mass activity (up to 25 times) for hydrogen evolution reaction. Results of extended x-ray absorption fine structure investigation and density functional theory calculation suggest that the active sites are associated with the lattice-confined Pt centers and the activated carbon (C)/nitrogen (N) atoms at the adjacency of the isolated Pt centers. This strategy may provide insights into constructing highly efficient single-atom catalysts for different energy-related applications.

Identifiers

PMID29372181
PMCPMC5775028
OpenAlexW2784507966

What OpenQuestion holds

Textmetadata
LicenceCC BY-NC
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.