ArticleACS applied materials & interfaces2018
Solvent Transport Behavior of Shear Aligned Graphene Oxide Membranes and Implications in Organic Solvent Nanofiltration.
Article in ACS applied materials & interfaces, 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 11 papers.
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Who cites it
11 citing papers in PubMed.
- Graphene-Oxide-Based Organic Solvent Filtration Membranes: Recent Progress and Perspectives.Chem & bio engineering · 2026Review
- Functionalized graphene oxide-based lamellar membranes for organic solvent nanofiltration applications.RSC advances · 2023Article
- Polymerization and Applications of Poly(methyl methacrylate)-Graphene Oxide Nanocomposites: A Review.ACS omega · 2022Review
- Recent Developments in Nanoporous Graphene Membranes for Organic Solvent Nanofiltration: A Short Review.Membranes · 2021Review
- Microscopically tuning the graphene oxide framework for membrane separations: a review.Nanoscale advances · 2021Review
- Catalytic Reduction of Graphene Oxide Membranes and Water Selective Channel Formation in Water-Alcohol Separations.Membranes · 2021Article
- Fabrication Techniques for Graphene Oxide-Based Molecular Separation Membranes: Towards Industrial Application.Nanomaterials (Basel, Switzerland) · 2021Review
- Ion and organic transport in Graphene oxide membranes: Model development to difficult water remediation applications.Journal of membrane science · 2020Article
- Selective molecular separation of lignin model compounds by reduced graphene oxide membranes from solvent-water mixture.Separation and purification technology · 2020Article
- Reduced graphene oxide-metal nanoparticle composite membranes for environmental separation and chloro-organic remediation.RSC advances · 2019Article
- Fabrication of Stacked Graphene Oxide Nanosheet Membranes Using Triethanolamine as a Crosslinker and Mild Reducing Agent for Water Treatment.Membranes · 2018Article
Corrections and comments
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Authors and funding
8 authors.
Funding
Abstract
Solvent transport in membranes composed of stacked sheets of graphene oxide (GO) with molecular scale channels and a complex arrangement of hydrophobic and hydrophilic domains is not well understood. Here, we observe that the interlayer space between GO sheets expands in different solvents without disturbing the membrane integrity and is typically larger in aqueous media compared to nonaqueous media. However, the membranes have a tighter molecule sieving feature in aqueous media as demonstrated by lower permeance and higher solute rejection arising from interfacial water layers "sticking" to charged polar groups. As a result of this polar interaction, the permeance of polar solvents in GO membrane scales inversely to the polarity of the solvent, which is contrary to other polymeric and ceramic hydrophilic membranes and also scales inversely to the viscosity of solvents as per continuum expectations. We highlight the extended solvent-handling space of GO membranes, such as in polar protic, polar aprotic, and nonpolar solvents, demonstrating versatility over a commercial nanofiltration membrane, and we predict exciting new applications in advanced separation engineering.
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