ArticleAngewandte Chemie (International ed. in English)2018
Photoinduced Pedalo-Type Motion in an Azodicarboxamide-Based Molecular Switch.
Article in Angewandte Chemie (International ed. in English), 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Exploring the Chemistry of the Mechanical Bond: Synthesis of a [2]Rotaxane through Multicomponent Reactions.Journal of chemical education · 2023Article
- Direct visual observation of pedal motion-dependent flexibility of single covalent organic frameworks.Nature communications · 2023Article
- Modus Operandi of a Pedalo-Type Molecular Switch: Insight from Dynamics and Theoretical Spectroscopy.Molecules (Basel, Switzerland) · 2023Article
- Atomistic Insight Into the Host-Guest Interaction of a Photoresponsive Metal-Organic Framework.Chemistry (Weinheim an der Bergstrasse, Germany) · 2020Article
- Recognition Selectivities of Lasso-Type Pseudo[1]rotaxane Based on a Mono-Ester-Functionalized Pillar[5]arene.Molecules (Basel, Switzerland) · 2019Article
- Modulation of Conformational Preferences of Heteroaromatic Ethers and Amides through Protonation and Ionization: Charge Effect.ChemistryOpen · 2019Article
- Tuning Electrochemical Bistability by Surface Area Blocking in the Cathodic Deposition of Copper.ACS omega · 2018Article
- Photoinduced Pedalo-Type Motion in an Azodicarboxamide-Based Molecular Switch.Angewandte Chemie (International ed. in English) · 2018Article
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Authors and funding
5 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Well-defined structural changes of molecular units that can be triggered by light are crucial for the development of photoactive functional materials. Herein, we report on a novel switch that has azodicarboxamide as its photo-triggerable element. Time-resolved UV-pump/IR probe spectroscopy in combination with quantum-chemical calculations shows that the azodicarboxamide functionality, in contrast to other azo-based chromophores, does not undergo trans-cis photoisomerization. Instead, a photoinduced pedalo-type motion occurs, which because of its volume-conserving properties enables the design of functional molecular systems with controllable motion in a confined space.
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