Evidence map›Paper›PMID 29119721›Full record

ArticleAngewandte Chemie (International ed. in English)2018

Integrated Transmission Electron and Single-Molecule Fluorescence Microscopy Correlates Reactivity with Ultrastructure in a Single Catalyst Particle.

Frank C Hendriks, Sajjad Mohammadian, Zoran Ristanović, Sam Kalirai, Florian Meirer, Eelco T C Vogt, Pieter C A Bruijnincx, Hans C Gerritsen, Bert M Weckhuysen

Abstract read
In one paragraph

Article in Angewandte Chemie (International ed. in English), 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 20 papers.

0numbers the graph read from it
0cells of the map it votes in
20citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

20 citing papers in PubMed.

  1. Review
  2. Review
  3. Nanoconfinement Effects in Electrocatalysis and Photocatalysis.Small (Weinheim an der Bergstrasse, Germany) · 2025
    Review
  4. Article
  5. Review
  6. Article
  7. Review
  8. Article
  9. Plastic Waste Conversion over a Refinery Waste Catalyst.Angewandte Chemie (International ed. in English) · 2021
    Article
  10. Article
  11. Article
  12. Article
  13. Article
  14. Article
  15. Article
  16. Article
  17. Article
  18. Staining a porous catalyst.Nature chemistry · 2019
    Article
  19. Communicating catalysts.Nature chemistry · 2018
    Article
  20. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

9 authors.

Frank C HendriksInorganic Chemistry and Catalysis, Debye Institute of Nanomaterials Science, Utrecht University, Universiteitsweg 99, 3584, CG, Utrecht, The Netherlands.
Sajjad MohammadianMolecular Biophysics, Department of Soft Condensed Matter and Biophysics, Science Faculty, Utrecht University, Princetonplein 1, 3584, CC, Utrecht, The Netherlands.
Zoran RistanovićInorganic Chemistry and Catalysis, Debye Institute of Nanomaterials Science, Utrecht University, Universiteitsweg 99, 3584, CG, Utrecht, The Netherlands.ORCID 0000-0001-9038-7066
Sam KaliraiInorganic Chemistry and Catalysis, Debye Institute of Nanomaterials Science, Utrecht University, Universiteitsweg 99, 3584, CG, Utrecht, The Netherlands.
Florian MeirerInorganic Chemistry and Catalysis, Debye Institute of Nanomaterials Science, Utrecht University, Universiteitsweg 99, 3584, CG, Utrecht, The Netherlands.ORCID 0000-0001-5581-5790
Eelco T C VogtInorganic Chemistry and Catalysis, Debye Institute of Nanomaterials Science, Utrecht University, Universiteitsweg 99, 3584, CG, Utrecht, The Netherlands.ORCID 0000-0003-4556-4283
Pieter C A BruijnincxInorganic Chemistry and Catalysis, Debye Institute of Nanomaterials Science, Utrecht University, Universiteitsweg 99, 3584, CG, Utrecht, The Netherlands.ORCID 0000-0001-8134-0530
Hans C GerritsenMolecular Biophysics, Department of Soft Condensed Matter and Biophysics, Science Faculty, Utrecht University, Princetonplein 1, 3584, CC, Utrecht, The Netherlands.
Bert M WeckhuysenInorganic Chemistry and Catalysis, Debye Institute of Nanomaterials Science, Utrecht University, Universiteitsweg 99, 3584, CG, Utrecht, The Netherlands.ORCID 0000-0001-5245-1426

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Establishing structure-activity relationships in complex, hierarchically structured nanomaterials, such as fluid catalytic cracking (FCC) catalysts, requires characterization with complementary, correlated analysis techniques. An integrated setup has been developed to perform transmission electron microscopy (TEM) and single-molecule fluorescence (SMF) microscopy on such nanostructured samples. Correlated structure-reactivity information was obtained for 100 nm thin, microtomed sections of a single FCC catalyst particle using this novel SMF-TEM high-resolution combination. High reactivity in a thiophene oligomerization probe reaction correlated well with TEM-derived zeolite locations, while matrix components, such as clay and amorphous binder material, were found not to display activity. Differences in fluorescence intensity were also observed within and between distinct zeolite aggregate domains, indicating that not all zeolite domains are equally active.

Indexed as

electron microscopyheterogeneous catalysissingle-molecule microscopystructure-activity relationshipszeolites

Identifiers

PMID29119721
PMCPMC5765468

What OpenQuestion holds

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LicenceCC BY-NC-ND
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Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.