ArticleACS nano2017
Pressure-Induced Melting of Confined Ice.
Article in ACS nano, 2017. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Navigating the Landscape of Dry Assembling Ordered Particle Structures: Can Solvents Become Obsolete?Small (Weinheim an der Bergstrasse, Germany) · 2024Review
- Ice-Enabled Transfer of Graphene on Copper Substrates Enhanced by Electric Field and CuAdvanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Photoconductivity Enhancement in Atomically Thin Molybdenum Disulfide through Local Doping from Confined Water.The journal of physical chemistry. C, Nanomaterials and interfaces · 2023Article
- High-Strain-Induced Local Modification of the Electronic Properties of VOACS applied electronic materials · 2022Article
- Structure, Properties, and Phase Transformations of Water Nanoconfined between Brucite-like Layers: The Role of Wall Surface Polarity.Materials (Basel, Switzerland) · 2022Article
- Tuning the Friction of Graphene on Mica by Alcohol Intercalation.Langmuir : the ACS journal of surfaces and colloids · 2019Article
- Universal Fermi-Level Pinning in Transition-Metal Dichalcogenides.The journal of physical chemistry. C, Nanomaterials and interfaces · 2019Article
- Influence of AFM Tip Temperature on THF Hydrate Stability: Theoretical Model and Numerical Simulation.Scanning · 2019Article
- Local Conduction in MoACS applied materials & interfaces · 2018Article
Corrections and comments
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Authors and funding
5 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The classic regelation experiment of Thomson in the 1850s deals with cutting an ice cube, followed by refreezing. The cutting was attributed to pressure-induced melting but has been challenged continuously, and only lately consensus emerged by understanding that compression shortens the O:H nonbond and lengthens the H-O bond simultaneously. This H-O elongation leads to energy loss and lowers the melting point. The hot debate survived well over 150 years, mainly due to a poorly defined heat exchange with the environment in the experiment. In our current experiment, we achieved thermal isolation from the environment and studied the fully reversible ice-liquid water transition for water confined between graphene and muscovite mica. We observe a transition from two-dimensional (2D) ice into a quasi-liquid phase by applying a pressure exerted by an atomic force microscopy tip. At room temperature, the critical pressure amounts to about 6 GPa. The transition is completely reversible: refreezing occurs when the applied pressure is lifted. The critical pressure to melt the 2D ice decreases with temperature, and we measured the phase coexistence line between 293 and 333 K. From a Clausius-Clapeyron analysis, we determine the latent heat of fusion of two-dimensional ice at 0.15 eV/molecule, being twice as large as that of bulk ice.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.