ArticleChemical science2017
Temporal switching of an amphiphilic self-assembly by a chemical fuel-driven conformational response.
Article in Chemical science, 2017. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 22 papers.
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Who cites it
22 citing papers in PubMed.
- Temporally Controlled Interconversion Between Suprasome and Supracube Structures to Regulate Catalytic Activities.Chemistry (Weinheim an der Bergstrasse, Germany) · 2026Article
- ATP-Regulated Formation of Transient Peptide Amphiphiles Superstructures.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- Non-equilibrium self-assembly for living matter-like properties.Nature reviews. Chemistry · 2024Review
- Construction of transient supramolecular polymers controlled by mass transfer in biphasic systems.Chemical science · 2022Article
- Temporally programmed polymer - solvent interactions using a chemical reaction network.Nature communications · 2022Article
- Room temperature charge-transfer phosphorescence from organic donor-acceptor Co-crystals.Chemical science · 2022Article
- Controlling the lifetime of cucurbit[8]uril based self-abolishing nanozymes.Chemical science · 2022Article
- Thiosquaramide-Based Supramolecular Polymers: Aromaticity Gain in a Switched Mode of Self-Assembly.Journal of the American Chemical Society · 2020Article
- Coupled Metabolic Cycles Allow Out-of-Equilibrium Autopoietic Vesicle Replication.Angewandte Chemie (International ed. in English) · 2020Article
- Transient dormant monomer states for supramolecular polymers with low dispersity.Nature communications · 2020Article
- Controlled synthesis of organic two-dimensional nanostructuresChemical science · 2020Article
- How Water in Aliphatic Solvents Directs the Interference of Chemical Reactivity in a Supramolecular System.Journal of the American Chemical Society · 2020Article
- Force generation by a propagating wave of supramolecular nanofibers.Nature communications · 2020Article
- Freeze the dynamicity: charge transfer complexation assisted control over the reaction pathway.Chemical science · 2019Article
- Bio-inspired temporal regulation of ion-transport in nanochannels.Nanoscale advances · 2019Article
- Chemical fuel-driven living and transient supramolecular polymerization.Nature communications · 2019Article
- Oscillations, travelling fronts and patterns in a supramolecular system.Nature nanotechnology · 2018Article
- A transient self-assembling self-replicator.Nature communications · 2018Article
- Bioinspired temporal supramolecular polymerization.RSC advances · 2018Review
- Feedback-Induced Temporal Control of "Breathing" Polymersomes To Create Self-Adaptive Nanoreactors.Journal of the American Chemical Society · 2018Article
Corrections and comments
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Authors and funding
4 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The spatial and temporal control of self-assemblies is the latest scientific hurdle in supramolecular chemistry which is inspired by the functioning of biological systems fueled by chemical signals. In this study, we work towards alleviating this scenario by employing a unique amphiphilic foldamer that operates under the effect of a chemical fuel. The conformational changes in the foldamer amplify into observable morphological changes in its amphiphilic assembly that are controlled by external molecular cues (fuel). We take advantage of this redox responsive foldamer to affect its conformation in a temporal manner by an enzymatic pathway. The temporal characteristics of the transient conformation/assembly can be modulated by varying the concentrations of the fuel and enzyme. We believe that such a design strategy can have positive consequences in designing molecular and supramolecular systems for future active, adaptive and autonomous materials.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.