ArticleNature materials2017
A map of high-mobility molecular semiconductors.
Article in Nature materials, 2017. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 59 papers.
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Who cites it
59 citing papers in PubMed.
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- Metallic charge transport in conjugated molecular bilayers.Nature electronics · 2026Article
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- Exploring the Interplay of Lattice Dynamics and Charge Transport in Organic Semiconductors: Progress Toward Rational Phonon Engineering.Angewandte Chemie (International ed. in English) · 2025Review
- Polymorph Screening and Investigation of Charge Transport of ditBuC6-BTBT.Crystal growth & design · 2025Article
- Crystal Engineering in Oligorylenes: The Quest for Optimized Crystal Packing and Enhanced Charge Transport.Crystal growth & design · 2025Article
- Two Isomeric Thienoacenes in Thin Films: Unveiling the Influence of Molecular Structure and Intermolecular Packing on Electronic Properties.The journal of physical chemistry. C, Nanomaterials and interfaces · 2024Article
- Thermoelectric transport in molecular crystals driven by gradients of thermal electronic disorder.Science advances · 2024Article
- On the importance of crystal structures for organic thin film transistors.Acta crystallographica. Section C, Structural chemistry · 2024Article
- Impact of hydrophilic side chains on the thin film transistor performance of a benzothieno-benzothiophene derivative.Materials advances · 2024Article
- Exciton Transport in the Nonfullerene Acceptor O-IDTBR from Nonadiabatic Molecular Dynamics.Journal of chemical theory and computation · 2024Article
- Accessing the electronic structure of liquid crystalline semiconductors with bottom-up electronic coarse-graining.Chemical science · 2024Article
- Grafting Electron-Accepting Fragments on [4]cyclo-2,7-carbazole Scaffold: Tuning the Structural and Electronic Properties of Nanohoops.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Structure-Property Relationships for the Electronic Applications of Bis-Adduct Isomers of Phenyl-CChemistry of materials : a publication of the American Chemical Society · 2024Article
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Authors and funding
5 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The charge mobility of molecular semiconductors is limited by the large fluctuation of intermolecular transfer integrals, often referred to as off-diagonal dynamic disorder, which causes transient localization of the carriers' eigenstates. Using a recently developed theoretical framework, we show here that the electronic structure of the molecular crystals determines its sensitivity to intermolecular fluctuations. We build a map of the transient localization lengths of high-mobility molecular semiconductors to identify what patterns of nearest-neighbour transfer integrals in the two-dimensional (2D) high-mobility plane protect the semiconductor from the effect of dynamic disorder and yield larger mobility. Such a map helps rationalizing the transport properties of the whole family of molecular semiconductors and is also used to demonstrate why common textbook approaches fail in describing this important class of materials. These results can be used to rapidly screen many compounds and design new ones with optimal transport characteristics.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.