ArticleChemical science2015
Synthesis of triazolium-based mono- and tris-branched [1]rotaxanes using a molecular transporter of dibenzo-24-crown-8.
Article in Chemical science, 2015. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
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Who cites it
12 citing papers in PubMed.
- Modulating the Swelling Behavior of Polymer Brushes via Interfacial Chemistry.Angewandte Chemie (International ed. in English) · 2026Article
- Skeletal Editing of Mechanically Interlocked Molecules: Nitrogen Atom Deletion from Crown Ether-Dibenzylammonium Rotaxanes.Journal of the American Chemical Society · 2024Article
- Diastereoselective synthesis of [1]rotaxanesChemical science · 2020Article
- Site-to-site peptide transport on a molecular platform using a small-molecule robotic arm.Chemical science · 2020Article
- Attempting to synthesize lasso peptides using high pressure.PloS one · 2020Article
- Active template rotaxane synthesis through the Ni-catalyzed cross-coupling of alkylzinc reagents with redox-active esters.Chemical science · 2019Article
- Synthesis of diamido-bridged bis-pillar[5]arenes and tris-pillar[5]arenes for construction of unique [1]rotaxanes and bis-[1]rotaxanes.Beilstein journal of organic chemistry · 2018Article
- How Secondary and Tertiary Amide Moieties are Molecular Stations for Dibenzo-24-crown-8 in [2]Rotaxane Molecular Shuttles?Molecules (Basel, Switzerland) · 2017Article
- Synthesis and stabilities of peptide-based [1]rotaxanes: molecular grafting onto lasso peptide scaffolds.Chemical science · 2017Article
- Radically promoted formation of a molecular lasso.Chemical science · 2017Article
- Formation of a series of stable pillar[5]arene-based pseudo[1]-rotaxanes and their [1]rotaxanes in the crystal state.Scientific reports · 2016Article
- One-pot synthesis of a [c2]daisy-chain-containing hetero[4]rotaxaneChemical science · 2016Article
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Authors and funding
4 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
We report a diverted route to [1]rotaxane and tris-branched [1]rotaxane that are devoid of any efficient template and which could not be obtained by classical straightforward strategies. The described chemical route relies on the utilization of a "macrocycle transporter", which is able first to bind a macrocycle, second to link temporarily a triazolium-containing molecular axle, and third to deliver the macrocycle around the new docked axle through molecular machinery in a [1]rotaxane structure. The extended encircled thread is eventually cleaved by an amine or a triamine to afford the triazolium-containing [1]rotaxanes, releasing at the same time, the macrocycle transporter as a recyclable species.
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