ArticleACS catalysis2017
Solvent Polarity-Induced Pore Selectivity in H-ZSM-5 Catalysis.
Article in ACS catalysis, 2017. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Microenvironment perturbations driving methanol low-temperature conversion over zeolite.Science advances · 2025Article
- Recent Advances in the Synthesis and Application of Monolayer 2D Metal-Organic Framework Nanosheets.Small science · 2024Article
- Hydrogen bonding to oxygen in siloxane bonds drives liquid phase adsorption of primary alcohols in high-silica zeolites.Materials horizons · 2023Article
- Unravelling Channel Structure-Diffusivity Relationships in Zeolite ZSM-5 at the Single-Molecule Level.Angewandte Chemie (International ed. in English) · 2022Article
- Maximizing sinusoidal channels of HZSM-5 for high shape-selectivity to p-xylene.Nature communications · 2019Article
- A Spectroscopic Study of Tautomeric Equilibrium of Salicylideneaniline in ZSM-5 Zeolites.Molecules (Basel, Switzerland) · 2019Article
- Reversible and Site-Dependent Proton-Transfer in Zeolites Uncovered at the Single-Molecule Level.Journal of the American Chemical Society · 2018Article
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Authors and funding
8 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Molecular-sized micropores of ZSM-5 zeolite catalysts provide spatial restrictions around catalytic sites that allow for shape-selective catalysis. However, the fact that ZSM-5 has two main pore systems with different geometries is relatively unexploited as a potential source of additional shape selectivity. Here, we use confocal laser-scanning microscopy to show that by changing the polarity of the solvent, the acid-catalyzed furfuryl alcohol oligomerization can be directed to selectively occur within either of two locations in the microporous network. This finding is confirmed for H-ZSM-5 particles with different Si/Al ratios and indicates a general trend for shape-selective catalytic reactions.
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