ArticleProceedings of the National Academy of Sciences of the United States of America2017
Diffusive dynamics during the high-to-low density transition in amorphous ice.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2017. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 54 papers.
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Who cites it
54 citing papers in PubMed.
- Unravelling Water Anomalies Using a Percolation Approach.ACS omega · 2026Article
- Time-resolved XPCS analysis across broad time-scales using multi-tau two-time correlations.Journal of synchrotron radiation · 2026Article
- MHz X-ray photon correlation spectroscopy using an acoustic levitator at the European XFEL.Journal of synchrotron radiation · 2025Article
- Multicomponent dynamics in amorphous ice studied using X-ray photon correlation spectroscopy at elevated pressure and cryogenic temperatures.Communications chemistry · 2025Article
- Nuclear quantum effects on glassy water under pressure: Vitrification and pressure-induced transformations.The Journal of chemical physics · 2024Article
- Supercritical density fluctuations and structural heterogeneity in supercooled water-glycerol microdroplets.Nature communications · 2024Article
- Complexity of confined water vitrification and its glass transition temperature.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- AI-NERD: Elucidation of relaxation dynamics beyond equilibrium through AI-informed X-ray photon correlation spectroscopy.Nature communications · 2024Article
- The laser pump X-ray probe system at LISA P08 PETRA III.Journal of synchrotron radiation · 2024Article
- High-pressure X-ray photon correlation spectroscopy at fourth-generation synchrotron sources.Journal of synchrotron radiation · 2024Article
- Water Potential from Adaptive Force Matching for Ice and Liquid with Revised Dispersion Predicts Supercooled Liquid Anomalies in Good Agreement with Two Independent Experimental Fits.The journal of physical chemistry. B · 2024Article
- A continuum of amorphous ices between low-density and high-density amorphous ice.Communications chemistry · 2024Article
- Improvement of ultra-small-angle XPCS with the Extremely Brilliant Source.Journal of synchrotron radiation · 2024Article
- Intrinsic Dynamics of Amorphous Ice Revealed by a Heterodyne Signal in X-ray Photon Correlation Spectroscopy Experiments.The journal of physical chemistry letters · 2023Article
- Lipid vesicle pools studied by passive X-ray microrheology.The European physical journal. E, Soft matter · 2023Article
- Calibrating TDDFT Calculations of the X-ray Emission Spectrum of Liquid Water: The Effects of Hartree-Fock Exchange.Journal of chemical theory and computation · 2023Article
- Pressure-induced nonmonotonic cross-over of steady relaxation dynamics in a metallic glass.Proceedings of the National Academy of Sciences of the United States of America · 2023Article
- Coherent X-ray Scattering Reveals Nanoscale Fluctuations in Hydrated Proteins.The journal of physical chemistry. B · 2023Article
- Glass Polymorphism in Hyperquenched Aqueous LiCl Solutions.The journal of physical chemistry. B · 2023Article
- Liquid-liquid phase separation in supercooled water from ultrafast heating of low-density amorphous ice.Nature communications · 2023Article
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Authors and funding
19 authors.
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Abstract
Water exists in high- and low-density amorphous ice forms (HDA and LDA), which could correspond to the glassy states of high- (HDL) and low-density liquid (LDL) in the metastable part of the phase diagram. However, the nature of both the glass transition and the high-to-low-density transition are debated and new experimental evidence is needed. Here we combine wide-angle X-ray scattering (WAXS) with X-ray photon-correlation spectroscopy (XPCS) in the small-angle X-ray scattering (SAXS) geometry to probe both the structural and dynamical properties during the high-to-low-density transition in amorphous ice at 1 bar. By analyzing the structure factor and the radial distribution function, the coexistence of two structurally distinct domains is observed at
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