ArticleScientific reports2017
Autocatalytic Time-Dependent Evolution of Metastable Two-Component Supramolecular Assemblies to Self-Sorted or Coassembled State.
Article in Scientific reports, 2017. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
What it found
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Who cites it
8 citing papers in PubMed.
- Cell-Like Synthetic Supramolecular Soft Materials Realized in Multicomponent, Non-/Out-of-Equilibrium Dynamic Systems.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Transient chirality inversion during racemization of a helical cobalt(III) complex.Proceedings of the National Academy of Sciences of the United States of America · 2022Article
- Control of seed formation allows two distinct self-sorting patterns of supramolecular nanofibers.Nature communications · 2020Article
- Transient dormant monomer states for supramolecular polymers with low dispersity.Nature communications · 2020Article
- Supramolecular double-stranded Archimedean spirals and concentric toroids.Nature communications · 2020Article
- Transient Supramolecular Hydrogels Formed by Aging-Induced Seeded Self-Assembly of Molecular Hydrogelators.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2020Article
- Living supramolecular polymerization based on reversible deactivation of a monomer by using a 'dummy' monomer.Chemical science · 2019Article
- Targetable Mechanical Properties by Switching between Self-Sorting and Co-assembly withChemNanoMat : chemistry of nanomaterials for energy, biology and more · 2018Article
Corrections and comments
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Authors and funding
3 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Despite substantial effort devoted in the history of supramolecular chemistry, synthetic supramolecular systems still lag behind biomolecular systems in terms of complexity and functionality. This is because biomolecular systems function in a multicomponent molecular network under out-of-equilibrium conditions. Here we report two-component supramolecular assemblies that are metastable and thus show time-dependent evolution. We found that the systems undergo either self-sorting or coassembly in time depending on the combination of components. Interestingly, this outcome, which had been previously achievable only under specific conditions, emerged from the two-component systems as a result of synergistic or reciprocal interplay between the coupled equilibria. We believe that this study sheds light on the similarity between synthetic and biomolecular systems and promotes better understanding of their intricate kinetic behaviors.
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Registered trials
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