ArticleNanomaterials (Basel, Switzerland)2017
Highly Enhanced Photoreductive Degradation of Polybromodiphenyl Ethers with g-C3N4/TiO2 under Visible Light Irradiation.
Article in Nanomaterials (Basel, Switzerland), 2017. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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4 citing papers in PubMed.
- TiOHeliyon · 2022Article
- Photocatalytic Performance and Degradation Pathway of Rhodamine B with TS-1/CNanomaterials (Basel, Switzerland) · 2020Article
- Enhanced UV-Visible Light Photocatalytic Activity by Constructing Appropriate Heterostructures between Mesopore TiO₂ Nanospheres and Sn₃O₄ Nanoparticles.Nanomaterials (Basel, Switzerland) · 2017Article
- Nanoscale in Photocatalysis.Nanomaterials (Basel, Switzerland) · 2017Article
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5 authors.
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Abstract
A series of high activity photocatalysts g-C3N4-TiO2 were synthesized by simple one-pot thermal transformation method and characterized by transmission electron microscopy (TEM), scanning electron microscopy (SEM), X-ray diffraction (XRD), X-ray photoelectron spectroscopy, Brunauer-Emmett-Teller (BET) surface area, and ultraviolet-visible diffuse reflectance spectroscopy (UV-Vis-DRS). The g-C3N4-TiO2 samples show highly improved photoreductive capability for the degradation of polybromodiphenyl ethers compared with g-C3N4 under visible light irradiation. Among all the hybrids, 0.02-C3N4-TiO2 with 2 wt % g-C3N4 loaded shows the highest reaction rate, which is 15 times as high as that in bare g-C3N4. The well-matched band gaps in heterojunction g-C3N4-TiO2 not only strengthen the absorption intensity, but also show more effective charge carrier separation, which results in the highly enhanced photoreductive performance under visible light irradiation. The trapping experiments show that holetrapping agents largely affect the reaction rate. The rate of electron accumulation in the conductive band is the rate-determining step in the degradation reaction. A possible photoreductive mechanism has been proposed.
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