ArticleACS nano2017
Cyanographene and Graphene Acid: Emerging Derivatives Enabling High-Yield and Selective Functionalization of Graphene.
Article in ACS nano, 2017. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 44 papers.
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44 citing papers in PubMed, 177 citations in OpenAlex.
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- Molecular Covalent Functionalization of Graphene and Its Derivatives: An Effective Strategy to Boost Electrocatalytic HER.ACS omega · 2025Review
- Aminosulfonated Graphene as a Catalyst for Efficient Production of Biodiesel from Fatty Acids and Crude Vegetable Oils.ChemSusChem · 2025Article
- E. coli and S. aureus resist silver nanoparticles via an identical mechanism, but through different pathways.Communications biology · 2024Article
- Real Time Tracking of Nanoconfined Water-Assisted Ion Transfer in Functionalized Graphene Derivatives Supercapacitor Electrodes.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Solvent Controlled Generation of Spin Active Polarons in Two-Dimensional Material under UV Light Irradiation.Journal of the American Chemical Society · 2024Article
- Graphene-Based Photodynamic Therapy and Overcoming Cancer Resistance Mechanisms: A Comprehensive Review.International journal of nanomedicine · 2024Review
- Linear-Structure Single-Atom Gold(I) Catalyst for Dehydrogenative Coupling of Organosilanes with Alcohols.ACS catalysis · 2023Article
- Lewis Acid Catalyzed Amide Bond Formation in Covalent Graphene-MOF Hybrids.The journal of physical chemistry. C, Nanomaterials and interfaces · 2023Article
- Graphene Amination towards Its Grafting by Antibodies for Biosensing Applications.Nanomaterials (Basel, Switzerland) · 2023Article
- Acidic graphene organocatalyst for the superior transformation of wastes into high-added-value chemicals.Nature communications · 2023Article
- A Multifunctional Integrated Metal-Free MRI Agent for Early Diagnosis of Oxidative Stress in a Mouse Model of Diabetic Cardiomyopathy.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Article
- Metal-free cysteamine-functionalized graphene alleviates mutual interferences in heavy metal electrochemical detection.Green chemistry : an international journal and green chemistry resource : GC · 2023Article
- One-pot carboxyl enrichment fosters water-dispersibility of reduced graphene oxide: a combined experimental and theoretical assessment.Nanoscale advances · 2023Article
- Graphene-Based Metal-Organic Framework Hybrids for Applications in Catalysis, Environmental, and Energy Technologies.Chemical reviews · 2022Review
- Coordination effects on the binding of late 3d single metal species to cyanographene.Physical chemistry chemical physics : PCCP · 2022Article
- Emerging graphene derivatives as active 2D coordination platforms for single-atom catalysts.Nanoscale · 2022Review
Corrections and comments
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Authors and funding
13 authors at 3 institutions in 2 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Efficient and selective methods for covalent derivatization of graphene are needed because they enable tuning of graphene's surface and electronic properties, thus expanding its application potential. However, existing approaches based mainly on chemistry of graphene and graphene oxide achieve only limited level of functionalization due to chemical inertness of the surface and nonselective simultaneous attachment of different functional groups, respectively. Here we present a conceptually different route based on synthesis of cyanographene via the controllable substitution and defluorination of fluorographene. The highly conductive and hydrophilic cyanographene allows exploiting the complex chemistry of -CN groups toward a broad scale of graphene derivatives with very high functionalization degree. The consequent hydrolysis of cyanographene results in graphene acid, a 2D carboxylic acid with pK
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