ArticleJournal of applied crystallography2017
Quantitative X-ray pair distribution function analysis of nanocrystalline calcium silicate hydrates: a contribution to the understanding of cement chemistry.
Article in Journal of applied crystallography, 2017. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 18 papers.
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Who cites it
18 citing papers in PubMed.
- Time-resolved synchrotron X-ray total scattering of alkali-activated materials with high and low calcium contents.Journal of synchrotron radiation · 2026Article
- Immobilization of CaPhysical chemistry chemical physics : PCCP · 2026Article
- Formation Mechanism and Resulting Physical Properties of Colloidal Calcium Silicate Hydrates.Langmuir : the ACS journal of surfaces and colloids · 2025Review
- Article
- Exploring the Potential of Nonclassical Crystallization Pathways to Advance Cementitious Materials.Chemical reviews · 2024Review
- Article
- Multi-step nucleation pathway of C-S-H during cement hydration from atomistic simulations.Nature communications · 2023Article
- Atomic-Level and Surface Structure of Calcium Silicate Hydrate Nanofoils.The journal of physical chemistry. C, Nanomaterials and interfaces · 2023Article
- Assessment of Pozzolanic Activity of Ground Scoria Rocks under Low- and High-Pressure (Autoclave) Steam Curing.Materials (Basel, Switzerland) · 2022Article
- Unveiling Non-isothermal Crystallization of CaO-AlInorganic chemistry · 2022Article
- Structure modeling and quantitative X-ray diffraction of C-(A)-S-H.Journal of applied crystallography · 2022Article
- An Atomistic Model Describing the Structure and Morphology of Cu-Doped C-S-H Hardening Accelerator Nanoparticles.Nanomaterials (Basel, Switzerland) · 2022Article
- Microstructure of CEM II/B-S Pastes Modified with Set Accelerating Admixtures.Materials (Basel, Switzerland) · 2021Article
- Article
- A Comparative Study of Experimental Configurations in Synchrotron Pair Distribution Function.Materials (Basel, Switzerland) · 2019Article
- Multiscale understanding of tricalcium silicate hydration reactions.Scientific reports · 2018Article
- Thermodynamic and crystallographic model for anion uptake by hydrated calcium aluminate (AFm): an example of molybdenum.Scientific reports · 2018Article
- Article
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10 authors.
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Abstract
The structural evolution of nanocrystalline calcium silicate hydrate (C-S-H) as a function of its calcium to silicon (Ca/Si) ratio has been probed using qualitative and quantitative X-ray atomic pair distribution function analysis of synchrotron X-ray scattering data. Whatever the Ca/Si ratio, the C-S-H structure is similar to that of tobermorite. When the Ca/Si ratio increases from ∼0.6 to ∼1.2, Si wollastonite-like chains progressively depolymerize through preferential omission of Si bridging tetrahedra. When the Ca/Si ratio approaches ∼1.5, nanosheets of portlandite are detected in samples aged for 1 d, while microcrystalline portlandite is detected in samples aged for 1 year. High-resolution transmission electron microscopy imaging shows that the tobermorite-like structure is maintained to Ca/Si > 3.
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