ArticleNature communications2017
Selective gating to vibrational modes through resonant X-ray scattering.
Article in Nature communications, 2017. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- Cuts through the manifold of molecular HProceedings of the National Academy of Sciences of the United States of America · 2022Article
- Vibrational resonant inelastic X-ray scattering in liquid acetic acid: a ruler for molecular chain lengths.Scientific reports · 2021Article
- Characterization of the soft X-ray spectrometer PEAXIS at BESSY II.Journal of synchrotron radiation · 2020Article
- Compatibility of quantitative X-ray spectroscopy with continuous distribution models of water at ambient conditions.Proceedings of the National Academy of Sciences of the United States of America · 2019Article
- Probing hydrogen bond strength in liquid water by resonant inelastic X-ray scattering.Nature communications · 2019Article
- Gradual collapse of nuclear wave functions regulated by frequency tuned X-ray scattering.Scientific reports · 2017Article
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Authors and funding
15 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The dynamics of fragmentation and vibration of molecular systems with a large number of coupled degrees of freedom are key aspects for understanding chemical reactivity and properties. Here we present a resonant inelastic X-ray scattering (RIXS) study to show how it is possible to break down such a complex multidimensional problem into elementary components. Local multimode nuclear wave packets created by X-ray excitation to different core-excited potential energy surfaces (PESs) will act as spatial gates to selectively probe the particular ground-state vibrational modes and, hence, the PES along these modes. We demonstrate this principle by combining ultra-high resolution RIXS measurements for gas-phase water with state-of-the-art simulations.
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