ArticleAngewandte Chemie (International ed. in English)2017
Backbone-Degradable Polymers Prepared by Chemical Vapor Deposition.
Article in Angewandte Chemie (International ed. in English), 2017. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed.
- Degradable Vinyl-Based Polymers by Radical Ring-Opening Polymerization: A User Guide.ACS polymers Au · 2026Article
- Localized gene delivery and enhanced cell-cell communication via bio-orthogonal polymer coatings.Regenerative engineering and translational medicine · 2025Article
- Systematic Studies into the Area Selectivity of Chemical Vapor Deposition Polymerization.ACS applied materials & interfaces · 2023Article
- BMP Gene-Immobilization to Dental Implants Enhances Bone Regeneration.Advanced materials interfaces · 2022Article
- Synthesis of degradable and chemically recyclable polymers using 4,4-disubstituted five-membered cyclic ketene hemiacetal ester (CKHE) monomers.Chemical science · 2021Article
- Vapor-deposited functional polymer thin films in biological applications.Journal of materials chemistry. B · 2020Review
- Materials and Orthopedic Applications for Bioresorbable Inductively Coupled Resonance Sensors.ACS applied materials & interfaces · 2020Article
- Regioselective Functionalization of [2.2]Paracyclophanes: Recent Synthetic Progress and Perspectives.Angewandte Chemie (International ed. in English) · 2020Review
- A Retro-biosynthesis-Based Route to Generate Pinene-Derived Polyesters.Chembiochem : a European journal of chemical biology · 2019Article
- Programmed Degradation of Hydrogels with a Double-Locked Domain.Angewandte Chemie (International ed. in English) · 2019Article
Corrections and comments
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Authors and funding
8 authors.
Funding
Abstract
Polymers prepared by chemical vapor deposition (CVD) polymerization have found broad acceptance in research and industrial applications. However, their intrinsic lack of degradability has limited wider applicability in many areas, such as biomedical devices or regenerative medicine. Herein, we demonstrate, for the first time, a backbone-degradable polymer directly synthesized via CVD. The CVD co-polymerization of [2.2]para-cyclophanes with cyclic ketene acetals, specifically 5,6-benzo-2-methylene-1,3-dioxepane (BMDO), results in well-defined, hydrolytically degradable polymers, as confirmed by FTIR spectroscopy and ellipsometry. The degradation kinetics are dependent on the ratio of ketene acetals to [2.2]para-cyclophanes as well as the hydrophobicity of the films. These coatings address an unmet need in the biomedical polymer field, as they provide access to a wide range of reactive polymer coatings that combine interfacial multifunctionality with degradability.
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Registered trials
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