ArticleScientific reports2016
Ultra-high electrochemical catalytic activity of MXenes.
Article in Scientific reports, 2016. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 14 papers.
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Who cites it
14 citing papers in PubMed.
- Facet-Selective Electrostatic Assembling of 2D MXene onto Anisotropic Single-Crystal Metal Oxides for Enhanced Photocatalysis.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Enhancing the Hydrogen Evolution Reaction Performance of TiChemphyschem : a European journal of chemical physics and physical chemistry · 2025Article
- Janus ScYCBrACS applied energy materials · 2024Article
- Review
- MXene Hybrid Nanosheet of WSACS omega · 2023Article
- Advancing MXene Electrocatalysts for Energy Conversion Reactions: Surface, Stoichiometry, and Stability.Angewandte Chemie (International ed. in English) · 2023Review
- Two-dimensional MXenes: recent emerging applications.RSC advances · 2022Review
- Substrate effect on hydrogen evolution reaction in two-dimensional MoScientific reports · 2022Article
- In Situ Growth of WNanomaterials (Basel, Switzerland) · 2022Article
- All-Optical Modulation Technology Based on 2D Layered Materials.Micromachines · 2022Review
- Double transition metal MXene (TiScientific reports · 2021Article
- Article
- Control of MXenes' electronic properties through termination and intercalation.Nature communications · 2019Article
- Antibacterial properties of electrospun TiRSC advances · 2018Article
Corrections and comments
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Authors and funding
1 author.
Funding
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Abstract
Cheap and abundant electrocatalysts for hydrogen evolution reactions (HER) have been widely pursued for their practical application in hydrogen-energy technologies. In this work, I present systematical study of the hydrogen evolution reactions on MXenes (Mo2X and W2X, X = C and N) based on density-functional-theory calculations. I find that their HER performances strongly depend on the composition, hydrogen adsorption configurations, and surface functionalization. I show that W2C monolayer has the best HER activity with near-zero overpotential at high hydrogen density among all of considered pure MXenes, and hydrogenation can efficiently enhance its catalytic performance in a wide range of hydrogen density further, while oxidization makes its activity reduced significantly. I further show that near-zero overpotential for HER on Mo2X monolayers can be achieved by oxygen functionalization. My calculations predict that surface treatment, such as hydrogenation and oxidization, is critical to enhance the catalytic performance of MXenes. I expect that MXenes with HER activity comparable to Pt in a wide range of hydrogen density can be realized by tuning composition and functionalizing, and promotes their applications into hydrogen-energy technologies.
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Registered trials
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