Evidence map›Paper›PMID 27572475›Full record

ArticleNature communications2016

Relating structure and composition with accessibility of a single catalyst particle using correlative 3-dimensional micro-spectroscopy.

Yijin Liu, Florian Meirer, Courtney M Krest, Samuel Webb, Bert M Weckhuysen

Abstract read
In one paragraph

Article in Nature communications, 2016. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 22 papers.

0numbers the graph read from it
0cells of the map it votes in
22citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

22 citing papers in PubMed.

  1. Article
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  8. Plastic Waste Conversion over a Refinery Waste Catalyst.Angewandte Chemie (International ed. in English) · 2021
    Article
  9. Review
  10. Article
  11. Article
  12. Article
  13. Article
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  15. Ion Concentration Polarization for Microparticle Mesoporosity Differentiation.Langmuir : the ACS journal of surfaces and colloids · 2019
    Article
  16. Article
  17. Article
  18. Article
  19. Article
  20. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

5 authors.

Yijin LiuStanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, California, 2575 Sand Hill Road, Menlo Park, California 94025, USA.
Florian MeirerInorganic Chemistry and Catalysis group, Debye Institute for Nanomaterials Science, Utrecht University, Utrecht, Universiteitsweg 99, 3584 CG Utrecht, The Netherlands.ORCID 0000-0001-5581-5790
Courtney M KrestStanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, California, 2575 Sand Hill Road, Menlo Park, California 94025, USA.
Samuel WebbStanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, California, 2575 Sand Hill Road, Menlo Park, California 94025, USA.
Bert M WeckhuysenInorganic Chemistry and Catalysis group, Debye Institute for Nanomaterials Science, Utrecht University, Utrecht, Universiteitsweg 99, 3584 CG Utrecht, The Netherlands.

Funding

X-ray Absorption Spectroscopy (XAS) pp.711-759P41GM103393 · NIGMS · STANFORD UNIVERSITY · PI HODGSON, KEITH O · 2012 to 2019
$30.6M
European Research CouncilNIGMS NIH HHS P41 GM103393
6 · The paper itself

Abstract

To understand how hierarchically structured functional materials operate, analytical tools are needed that can reveal small structural and chemical details in large sample volumes. Often, a single method alone is not sufficient to get a complete picture of processes happening at multiple length scales. Here we present a correlative approach combining three-dimensional X-ray imaging techniques at different length scales for the analysis of metal poisoning of an individual catalyst particle. The correlative nature of the data allowed establishing a macro-pore network model that interprets metal accumulations as a resistance to mass transport and can, by tuning the effect of metal deposition, simulate the response of the network to a virtual ageing of the catalyst particle. The developed approach is generally applicable and provides an unprecedented view on dynamic changes in a material's pore space, which is an essential factor in the rational design of functional porous materials.

Indexed as

CatalysisFluorescenceImaging, Three-DimensionalMaterials TestingMetalsMicroscopyModels, ChemicalParticle SizePorositySpectrum AnalysisSynchrotronsX-Ray MicrotomographyMetals

Identifiers

PMID27572475
PMCPMC5013607

What OpenQuestion holds

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LicenceCC BY
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Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.