ArticleNature communications2016
A possible four-phase coexistence in a single-component system.
Article in Nature communications, 2016. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Persistent homology elucidates hierarchical structures responsible for mechanical properties in covalent amorphous solids.Nature communications · 2025Article
- Article
- Multiphase Coexistence in Binary Hard Colloidal Mixtures: Predictions from a Simple Algebraic Theory.The journal of physical chemistry letters · 2023Article
- Revealing thermally-activated nucleation pathways of diffusionless solid-to-solid transition.Nature communications · 2021Article
- Water-like anomalies as a function of tetrahedrality.Proceedings of the National Academy of Sciences of the United States of America · 2018Article
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Authors and funding
3 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
For different phases to coexist in equilibrium at constant temperature T and pressure P, the condition of equal chemical potential μ must be satisfied. This condition dictates that, for a single-component system, the maximum number of phases that can coexist is three. Historically this is known as the Gibbs phase rule, and is one of the oldest and venerable rules of thermodynamics. Here we make use of the fact that, by varying model parameters, the Gibbs phase rule can be generalized so that four phases can coexist even in single-component systems. To systematically search for the quadruple point, we use a monoatomic system interacting with a Stillinger-Weber potential with variable tetrahedrality. Our study indicates that the quadruple point provides flexibility in controlling multiple equilibrium phases and may be realized in systems with tunable interactions, which are nowadays feasible in several soft matter systems such as patchy colloids.
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Registered trials
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