ArticleNature communications2016
Visualization of anisotropic-isotropic phase transformation dynamics in battery electrode particles.
Article in Nature communications, 2016. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 21 papers.
What it found
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Who cites it
21 citing papers in PubMed.
- Multidimensional Tracking and Clustering of Electrochemical Reactions in the Positive Electrode of Lithium-Ion Batteries via Operando X‑ray Nanoscale Chemical Imaging.Chemical & biomedical imaging · 2026Article
- Image registration for accurate electrode deformation analysis in operando microscopy of battery materials.Journal of synchrotron radiation · 2025Article
- Image registration for in situ X-ray nano-imaging of a composite battery cathode with deformation.Journal of synchrotron radiation · 2024Article
- Nanoscale chemical imaging with structured X-ray illumination.Proceedings of the National Academy of Sciences of the United States of America · 2023Article
- Effective transport network driven by tortuosity gradient enables high-electrochem-active solid-state batteries.National science review · 2023Article
- Synchrotron radiation basedChemical science · 2023Review
- Quantificational 4D Visualization of Industrial Electrodeposition.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2021Article
- Probing Kinetics of Water-in-Salt Aqueous Batteries with Thick Porous Electrodes.ACS central science · 2021Article
- Evolution and expansion of Li concentration gradient during charge-discharge cycling.Nature communications · 2021Article
- Sparse ab initio x-ray transmission spectrotomography for nanoscopic compositional analysis of functional materials.Science advances · 2021Article
- Depth-dependent valence stratification driven by oxygen redox in lithium-rich layered oxide.Nature communications · 2020Article
- Insights into interfacial effect and local lithium-ion transport in polycrystalline cathodes of solid-state batteries.Nature communications · 2020Article
- Machine-learning-revealed statistics of the particle-carbon/binder detachment in lithium-ion battery cathodes.Nature communications · 2020Article
- Quantifying redox heterogeneity in single-crystalline LiCoOJournal of synchrotron radiation · 2020Article
- Systems-level investigation of aqueous batteries for understanding the benefit of water-in-salt electrolyte by synchrotron nanoimaging.Science advances · 2020Article
- Probing the reversibility and kinetics of LiChemical science · 2019Article
- Propagation topography of redox phase transformations in heterogeneous layered oxide cathode materials.Nature communications · 2018Article
- X-ray physico-chemical imaging during activation of cobalt-based Fischer-Tropsch synthesis catalysts.Philosophical transactions. Series A, Mathematical, physical, and engineering sciences · 2018Article
- Two-dimensional lithium diffusion behavior and probable hybrid phase transformation kinetics in olivine lithium iron phosphate.Nature communications · 2017Article
- Phase transformation mechanism in lithium manganese nickel oxide revealed by single-crystal hard X-ray microscopy.Nature communications · 2017Article
Corrections and comments
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Authors and funding
5 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Anisotropy, or alternatively, isotropy of phase transformations extensively exist in a number of solid-state materials, with performance depending on the three-dimensional transformation features. Fundamental insights into internal chemical phase evolution allow manipulating materials with desired functionalities, and can be developed via real-time multi-dimensional imaging methods. Here, we report a five-dimensional imaging method to track phase transformation as a function of charging time in individual lithium iron phosphate battery cathode particles during delithiation. The electrochemically driven phase transformation is initially anisotropic with a preferred boundary migration direction, but becomes isotropic as delithiation proceeds further. We also observe the expected two-phase coexistence throughout the entire charging process. We expect this five-dimensional imaging method to be broadly applicable to problems in energy, materials, environmental and life sciences.
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Registered trials
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