Evidence map›Paper›PMID 26804546›Full record

ArticleNature communications2016

Mapping multidimensional electronic structure and ultrafast dynamics with single-element detection and compressive sensing.

Austin P Spencer, Boris Spokoyny, Supratim Ray, Fahad Sarvari, Elad Harel

Abstract read
In one paragraph

Article in Nature communications, 2016. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.

0numbers the graph read from it
0cells of the map it votes in
4citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

4 citing papers in PubMed.

  1. Article
  2. Article
  3. Article
  4. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

5 authors.

Austin P SpencerDepartment of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinosis 60208, USA.
Boris SpokoynyDepartment of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinosis 60208, USA.
Supratim RayDepartment of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinosis 60208, USA.
Fahad SarvariDepartment of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinosis 60208, USA.
Elad HarelDepartment of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinosis 60208, USA.

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Compressive sensing allows signals to be efficiently captured by exploiting their inherent sparsity. Here we implement sparse sampling to capture the electronic structure and ultrafast dynamics of molecular systems using phase-resolved 2D coherent spectroscopy. Until now, 2D spectroscopy has been hampered by its reliance on array detectors that operate in limited spectral regions. Combining spatial encoding of the nonlinear optical response and rapid signal modulation allows retrieval of state-resolved correlation maps in a photosynthetic protein and carbocyanine dye. We report complete Hadamard reconstruction of the signals and compression factors as high as 10, in good agreement with array-detected spectra. Single-point array reconstruction by spatial encoding (SPARSE) Spectroscopy reduces acquisition times by about an order of magnitude, with further speed improvements enabled by fast scanning of a digital micromirror device. We envision unprecedented applications for coherent spectroscopy using frequency combs and super-continua in diverse spectral regions.

Identifiers

PMID26804546
PMCPMC4737750

What OpenQuestion holds

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LicenceCC BY
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Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.