ArticleStructural dynamics (Melville, N.Y.)2016
Activation of coherent lattice phonon following ultrafast molecular spin-state photo-switching: A molecule-to-lattice energy transfer.
Article in Structural dynamics (Melville, N.Y.), 2016. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed.
- The Part and the Whole: Field-Dependent THz-EPR Spectroscopy Probes Lattice-Dependent Electronic Structure in Iron(II) Spin Crossover.Angewandte Chemie (International ed. in English) · 2026Article
- Elucidating the Transition Kernel and Anharmonic Coupling in the Spin-crossover Process of a [FeAngewandte Chemie (International ed. in English) · 2026Article
- Capturing ultrafast molecular motions and lattice dynamics in spin crossover film using femtosecond diffraction methods.Nature communications · 2025Article
- Dynamics of Spin Crossover Molecular Complexes.Nanomaterials (Basel, Switzerland) · 2022Review
- Direct observation of nuclear reorganization driven by ultrafast spin transitions.Nature communications · 2020Article
- Perspective: Opportunities for ultrafast science at SwissFEL.Structural dynamics (Melville, N.Y.) · 2017Article
- Comparison of structural dynamics and coherence of d-d and MLCT light-induced spin state trapping.Chemical science · 2017Article
- Coherent ultrafast lattice-directed reaction dynamics of triiodide anion photodissociation.Nature chemistry · 2017Article
- Time-resolved X-ray spectroscopies of chemical systems: New perspectives.Structural dynamics (Melville, N.Y.) · 2016Article
- Preface to Special Topic: Invited Papers of the 3rd International Conference on Ultrafast Structural Dynamics.Structural dynamics (Melville, N.Y.) · 2016Article
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Authors and funding
9 authors.
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Abstract
We combine ultrafast optical spectroscopy with femtosecond X-ray absorption to study the photo-switching dynamics of the [Fe(PM-AzA)2(NCS)2] spin-crossover molecular solid. The light-induced excited spin-state trapping process switches the molecules from low spin to high spin (HS) states on the sub-picosecond timescale. The change of the electronic state (<50 fs) induces a structural reorganization of the molecule within 160 fs. This transformation is accompanied by coherent molecular vibrations in the HS potential and especially a rapidly damped Fe-ligand breathing mode. The time-resolved studies evidence a delayed activation of coherent optical phonons of the lattice surrounding the photoexcited molecules.
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