ArticleScientific reports2015
A hierarchical view on material formation during pulsed-laser synthesis of nanoparticles in liquid.
Article in Scientific reports, 2015. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 15 papers.
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Who cites it
15 citing papers in PubMed.
- Time-Resolved Dynamics of Laser Ablation in Liquid with Gas-Evolving Additives: Toward Molding the Atomic Structure of Nonequilibrium Nanoalloys.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Morphology and properties of pyrite nanoparticles obtained by pulsed laser ablation in liquid and thin films for photodetection.Beilstein journal of nanotechnology · 2025Article
- Laser processing in liquids: insights into nanocolloid generation and thin film integration for energy, photonic, and sensing applications.Beilstein journal of nanotechnology · 2025Review
- State of the Art in Gold Nanoparticle Synthesisation via Pulsed Laser Ablation in Liquid and Its Characterisation for Molecular Imaging: A Review.Materials (Basel, Switzerland) · 2022Review
- Pump-probe X-ray holographic imaging of laser-induced cavitation bubbles with femtosecond FEL pulses.Nature communications · 2021Article
- How the Physicochemical Properties of the Bulk Material Affect the Ablation Crater Profile, Mass Balance, and Bubble Dynamics During Single-Pulse, Nanosecond Laser Ablation in Water.Chemistry (Weinheim an der Bergstrasse, Germany) · 2021Article
- Laser Synthesis and Microfabrication of Micro/Nanostructured Materials Toward Energy Conversion and Storage.Nano-micro letters · 2021Review
- The influence of the fluid nature on femtosecond laser ablation properties of a SiONanoscale advances · 2020Article
- Doping nanoparticles using pulsed laser ablation in a liquid containing the doping agent.Nanoscale advances · 2019Article
- Explosives sensing using Ag-Cu alloy nanoparticles synthesized by femtosecond laser ablation and irradiation.RSC advances · 2019Article
- Magnetic Fe@FeONanomaterials (Basel, Switzerland) · 2018Article
- Two mechanisms of nanoparticle generation in picosecond laser ablation in liquids: the origin of the bimodal size distribution.Nanoscale · 2018Article
- BiACS omega · 2017Article
- Generation of Subsurface Voids, Incubation Effect, and Formation of Nanoparticles in Short Pulse Laser Interactions with Bulk Metal Targets in Liquid: Molecular Dynamics Study.The journal of physical chemistry. C, Nanomaterials and interfaces · 2017Article
- In situ decoration of graphene sheets with gold nanoparticles synthetized by pulsed laser ablation in liquids.Scientific reports · 2016Article
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Authors and funding
8 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Pulsed-laser assisted nanoparticle synthesis in liquids (PLAL) is a versatile tool for nanoparticle synthesis. However, fundamental aspects of structure formation during PLAL are presently poorly understood. We analyse the spatio-temporal kinetics during PLAL by means of fast X-ray radiography (XR) and scanning small-angle X-ray scattering (SAXS), which permits us to probe the process on length scales from nanometers to millimeters with microsecond temporal resolution. We find that the global structural evolution, such as the dynamics of the vapor bubble can be correlated to the locus and evolution of silver nanoparticles. The bubble plays an important role in particle formation, as it confines the primary particles and redeposits them to the substrate. Agglomeration takes place for the confined particles in the second bubble. Additionally, upon the collapse of the second bubble a jet of confined material is ejected perpendicularly to the surface. We hypothesize that these kinetics influence the final particle size distribution and determine the quality of the resulting colloids, such as polydispersity and modality through the interplay between particle cloud compression and particle release into the liquid.
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Registered trials
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