ArticleSmall (Weinheim an der Bergstrasse, Germany)2015
A Thermodynamics Model for the Emergence of a Stripe-like Binary SAM on a Nanoparticle Surface.
Article in Small (Weinheim an der Bergstrasse, Germany), 2015. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- Understanding the Two-Dimensional Mixing Behavior of 1-Naphthalenethiol and Octanethiol.The journal of physical chemistry. C, Nanomaterials and interfaces · 2023Article
- Inhibition of Amyloid Aggregation and Toxicity with Janus Iron Oxide Nanoparticles.Chemistry of materials : a publication of the American Chemical Society · 2021Article
- Mass spectrometry and Monte Carlo method mapping of nanoparticle ligand shell morphology.Nature communications · 2018Article
- Quantitative 3D determination of self-assembled structures on nanoparticles using small angle neutron scattering.Nature communications · 2018Article
- Gold nanoparticles with patterned surface monolayers for nanomedicine: current perspectives.European biophysics journal : EBJ · 2017Review
- Brushed polyethylene glycol and phosphorylcholine for grafting nanoparticles against protein binding.Polymer chemistry · 2016Article
Corrections and comments
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Authors and funding
4 authors.
Funding
Abstract
It has been under debate if a self-assembled monolayer (SAM) with two immiscible ligands of different chain lengths and/or bulkiness can form a stripe-like pattern on a nanoparticle (NP) surface. The entropic gain upon such pattern formation due to difference in chain lengths and/or bulkiness has been proposed as the driving force in literature. Using atomistic discrete molecular dynamics simulations it is shown that stripe-like pattern could indeed emerge, but only for a subset of binary SAM systems. In addition to entropic contributions, the formation of a striped pattern also strongly depends upon interligand interactions governed by the physicochemical properties of the ligand constituents. Due to the interplay between entropy and enthalpy, a binary SAM system can be categorized into three different types depending on whether and under what condition a striped pattern can emerge. The results help clarify the ongoing debate and our proposed principle can aid in the engineering of novel binary SAMs on a NP surface.
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Registered trials
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