ArticleNature communications2015
Supramolecular block copolymers by kinetically controlled co-self-assembly of planar and core-twisted perylene bisimides.
Article in Nature communications, 2015. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 59 papers.
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Who cites it
59 citing papers in PubMed.
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- Tunable Thermally Activated Delayed Fluorescence from Supramolecular Polymers Toward Application in Aqueous Media.Angewandte Chemie (International ed. in English) · 2025Article
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- Electronically and geometrically complementary perylenediimides for kinetically controlled supramolecular copolymers.Chemical science · 2024Article
- Supramolecular copolymerization of hydrophobic and hydrophilic monomers in liquid crystalline media.Chemical science · 2024Article
- Therapeutic Supramolecular Polymers: Designs and Applications.Progress in polymer science · 2024Article
- Supramolecular alternating copolymers with highly efficient fluorescence resonance energy transfer.Chemical science · 2023Article
- Energy Landscapes of Supramolecular Peptide-Drug Conjugates Directed by Linker Selection and Drug Topology.ACS nano · 2022Article
- Anti-cooperative Self-Assembly with Maintained Emission Regulated by Conformational and Steric Effects.Angewandte Chemie (International ed. in English) · 2022Article
- Hierarchical self-assembly of aromatic peptide conjugates into supramolecular polymers: it takes two to tango.Chemical science · 2022Review
- Supramolecular polymerization of electronically complementary linear motifs: anti-cooperativity by attenuated growth.Chemical science · 2021Article
- Non-uniform Photoinduced Unfolding of Supramolecular Polymers Leading to Topological Block Nanofibers.Angewandte Chemie (International ed. in English) · 2021Article
- Unraveling the Complexity of Supramolecular Copolymerization Dictated by Triazine-Benzene Interactions.Journal of the American Chemical Society · 2021Article
- Exploring the Potential of Benzene-1,3,5-tricarboxamide Supramolecular Polymers as Biomaterials.Biomacromolecules · 2020Article
- Long-Lived Charge-Transfer State from B-N Frustrated Lewis Pairs Enchained in Supramolecular Copolymers.Journal of the American Chemical Society · 2020Article
- Homopolymer self-assembly of poly(propylene sulfone) hydrogels via dynamic noncovalent sulfone-sulfone bonding.Nature communications · 2020Article
- Control of seed formation allows two distinct self-sorting patterns of supramolecular nanofibers.Nature communications · 2020Article
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Authors and funding
4 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
New synthetic methodologies for the formation of block copolymers have revolutionized polymer science within the last two decades. However, the formation of supramolecular block copolymers composed of alternating sequences of larger block segments has not been realized yet. Here we show by transmission electron microscopy (TEM), 2D NMR and optical spectroscopy that two different perylene bisimide dyes bearing either a flat (A) or a twisted (B) core self-assemble in water into supramolecular block copolymers with an alternating sequence of (AmBB)n. The highly defined ultralong nanowire structure of these supramolecular copolymers is entirely different from those formed upon self-assembly of the individual counterparts, that is, stiff nanorods (A) and irregular nanoworms (B), respectively. Our studies further reveal that the as-formed supramolecular block copolymer constitutes a kinetic self-assembly product that transforms into thermodynamically more stable self-sorted homopolymers upon heating.
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