ArticleNature communications2014
Quantum yield and excitation rate of single molecules close to metallic nanostructures.
Article in Nature communications, 2014. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 35 papers.
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Who cites it
35 citing papers in PubMed.
- Three-dimensional plasmonic nanopores for DNA-PAINT and dual-material Au/Si architectures.Journal of nanobiotechnology · 2026Article
- High-Throughput Fabrication of Zero-Mode Waveguide Nanoaperture Arrays with Sol-Gel Nanoimprint Lithography for Enhanced Single Molecule Fluorescence Detection.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Insights on using plastic-based dual in-plane nanopore sensors for differentiation and shape determinations of single protein molecules.Scientific reports · 2025Article
- Harnessing the Power of Plasmonics forACS photonics · 2025Review
- Multiple Scattering-Enhanced Fluorescence Within Randomly Oriented Low-Index Polymer Nanofiber Sensors.Biosensors · 2025Article
- An overview on plasmon-enhanced photoluminescence via metallic nanoantennas.Nanophotonics (Berlin, Germany) · 2024Article
- Hexagonal Plasmonic Arrays for High-Throughput Multicolor Single-Molecule Studies.ACS applied materials & interfaces · 2024Article
- Confined semiconducting polymers with boosted NIR light-triggered HChemical science · 2024Article
- Article
- Strategies for Overcoming the Single-Molecule Concentration Barrier.ACS measurement science au · 2023Review
- Excitation Intensity-Dependent Quantum Yield of Semiconductor Nanocrystals.The journal of physical chemistry letters · 2023Article
- Visualization of Polymer-Surfactant Interaction by Dual-Emissive Gold Nanocluster Labeling.Biosensors · 2022Article
- Electromechanical Photophysics of GFP Packed Inside Viral Protein Cages Probed by Force-Fluorescence Hybrid Single-Molecule Microscopy.Small (Weinheim an der Bergstrasse, Germany) · 2022Article
- Gold Ion Beam Milled Gold Zero-Mode Waveguides.Nanomaterials (Basel, Switzerland) · 2022Article
- DNA Origami Nanoantennas for Fluorescence Enhancement.Accounts of chemical research · 2021Article
- Recent advances in plasmonic nanocavities for single-molecule spectroscopy.Nanoscale advances · 2021Review
- Absolute quantum yield measurements of fluorescent proteins using a plasmonic nanocavity.Communications biology · 2020Article
- Mixed metal zero-mode guides (ZMWs) for tunable fluorescence enhancement.Nanoscale advances · 2020Article
- Review
- Unveiling the radiative local density of optical states of a plasmonic nanocavity by STM.Nature communications · 2020Article
Corrections and comments
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Authors and funding
6 authors.
Funding
Abstract
The interaction of dyes and metallic nanostructures strongly affects the fluorescence and can lead to significant fluorescence enhancement at plasmonic hot spots, but also to quenching. Here we present a method to distinguish the individual contributions to the changes of the excitation, radiative and non-radiative rate and use this information to determine the quantum yields for single molecules. The method is validated by precisely placing single fluorescent dyes with respect to gold nanoparticles as well as with respect to the excitation polarization using DNA origami nanostructures. Following validation, measurements in zeromode waveguides reveal that suppression of the radiative rate and enhancement of the non-radiative rate lead to a reduced quantum yield. Because the method exploits the intrinsic blinking of dyes, it can generally be applied to fluorescence measurements in arbitrary nanophotonic environments.
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Registered trials
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