ArticleAngewandte Chemie (International ed. in English)2014
A simple and highly effective ligand system for the copper(I)-mediated assembly of rotaxanes.
Article in Angewandte Chemie (International ed. in English), 2014. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Triple Self-Sorting in Constitutional Dynamic Networks: Parallel Generation of Imine-Based CuAngewandte Chemie (International ed. in English) · 2020Article
- Self-sorting of two imine-based metal complexes: balancing kinetics and thermodynamics in constitutional dynamic networks.Chemical science · 2019Article
- Differential metal-binding properties of dynamic acylhydrazone polymers and their sensing applications.Royal Society open science · 2017Article
- Macrocyclic shape-persistency of cyclo[6]aramide results in enhanced multipoint recognition for the highly efficient template-directed synthesis of rotaxanes.Chemical science · 2017Article
- High yielding synthesis of 2,2'-bipyridine macrocycles, versatile intermediates in the synthesis of rotaxanes.Chemical science · 2016Article
- Fuel-Controlled Reassembly of Metal-Organic Architectures.ACS central science · 2015Article
- Competitive formation of homocircuit [3]rotaxanes in synthetically useful yields in the bipyridine-mediated active template CuAAC reaction.Chemical science · 2015Article
Corrections and comments
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Authors and funding
4 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
A [2]rotaxane was produced through the assembly of a picolinaldehyde, an amine, and a bipyridine macrocycle around a Cu(I) template by imine bond formation in close-to-quantitative yield. An analogous [3]rotaxane is obtained in excellent yield by replacing the amine with a diamine, thus showing the suitability of the system for the construction of higher order interlocked structures. The rotaxanes are formed within a few minutes simply through mixing the components in solution at room temperature and they can be isolated through removal of the solvent or precipitation.
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