Evidence map›Paper›PMID 25177427›Full record

ArticleThe journal of physical chemistry letters2014

Stimulated Raman Spectroscopy with Entangled Light: Enhanced Resolution and Pathway Selection.

Konstantin E Dorfman, Frank Schlawin, Shaul Mukamel

Abstract read
In one paragraph

Article in The journal of physical chemistry letters, 2014. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.

0numbers the graph read from it
0cells of the map it votes in
9citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

9 citing papers in PubMed.

  1. Quantum-enhanced coherent Raman spectroscopy with broadband squeezed-light detection.Proceedings of the National Academy of Sciences of the United States of America · 2026
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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

3 authors.

Konstantin E DorfmanDepartment of Chemistry, University of California , Irvine, California 92697-2025, United States.
Frank SchlawinDepartment of Chemistry, University of California , Irvine, California 92697-2025, United States ; Physikalisches Institut, Albert-Ludwigs-Universität Freiburg , Hermann-Herder-Straße 3, 79104 Freiburg, Germany.
Shaul MukamelDepartment of Chemistry, University of California , Irvine, California 92697-2025, United States.

Funding

Multidimensional Femtosecond Correlation Spectroscopic Probes of BiomoleculesR01GM059230 · NIGMS · UNIVERSITY OF ROCHESTER · PI MUKAMEL, SHAUL · 2001 to 2013
$3.2M
NIGMS NIH HHS R01 GM059230
6 · The paper itself

Abstract

We propose a novel femtosecond stimulated Raman spectroscopy (FSRS) technique that combines entangled photons with interference detection to select matter pathways and enhance the resolution. Following photoexcitation by an actinic pump, the measurement uses a pair of broad-band entangled photons; one (signal) interacts with the molecule and together with a third narrow-band pulse induces the Raman process. The other (idler) photon provides a reference for the coincidence measurement. This interferometric photon coincidence counting detection allows one to separately measure the Raman gain and loss signals, which is not possible with conventional probe transmission detection. Entangled photons further provide a unique temporal and spectral detection window that can better resolve fast excited-state dynamics compared to classical and correlated disentangled states of light.

Identifiers

PMID25177427
PMCPMC4141681

What OpenQuestion holds

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.