ArticleScientific reports2014
Critical behavior of a water monolayer under hydrophobic confinement.
Article in Scientific reports, 2014. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Unravelling Water Anomalies Using a Percolation Approach.ACS omega · 2026Article
- The Rose Model of Water: Linking Theory and Simulation.Entropy (Basel, Switzerland) · 2026Article
- Snowflake Model of Water: A Fast Approach for Calculation of Structural Properties of Liquid Water.Journal of chemical theory and computation · 2025Article
- Advances in the study of supercooled water.The European physical journal. E, Soft matter · 2021Review
- Article
- Hierarchy of anomalies in the two-dimensional Mercedes-Benz model of water.Physical review. E · 2018Article
- Phase diagram of hard squares in slit confinement.Scientific reports · 2018Article
- Dissecting the Forces that Dominate Dimerization of the Nucleotide Binding Domains of ABCB1.Biophysical journal · 2018Article
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Authors and funding
2 authors.
Funding
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Abstract
The properties of water can have a strong dependence on the confinement. Here, we consider a water monolayer nanoconfined between hydrophobic parallel walls under conditions that prevent its crystallization. We investigate, by simulations of a many-body coarse-grained water model, how the properties of the liquid are affected by the confinement. We show, by studying the response functions and the correlation length and by performing finite-size scaling of the appropriate order parameter, that at low temperature the monolayer undergoes a liquid-liquid phase transition ending in a critical point in the universality class of the two-dimensional (2D) Ising model. Surprisingly, by reducing the linear size L of the walls, keeping the walls separation h constant, we find a 2D-3D crossover for the universality class of the liquid-liquid critical point for L=h ≃ 50, i.e. for a monolayer thickness that is small compared to its extension. This result is drastically different from what is reported for simple liquids, where the crossover occurs for L=h ≃ 5, and is consistent with experimental results and atomistic simulations. We shed light on these findings showing that they are a consequence of the strong cooperativity and the low coordination number of the hydrogen bond network that characterizes water.
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