ArticleNature2013
Stimulated X-ray emission for materials science.
Article in Nature, 2013. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 23 papers.
What it found
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Who cites it
23 citing papers in PubMed, 116 citations in OpenAlex.
- Multiplet lines in seeded stimulated MnPhysical review applied · 2026Article
- Stimulated X-ray emission spectroscopy.Photosynthesis research · 2024Review
- Electron population dynamics in resonant non-linear x-ray absorption in nickel at a free-electron laser.Structural dynamics (Melville, N.Y.) · 2023Article
- Two-dimensional Kβ-Kα fluorescence spectrum by nonlinear resonant inelastic X-ray scattering.Nature communications · 2023Article
- Seeded stimulated X-ray emission at 5.9 keV.Optica · 2023Article
- Observation of Seeded Mn Kβ Stimulated X-Ray Emission Using Two-Color X-Ray Free-Electron Laser Pulses.Physical review letters · 2020Article
- Narrow-band hard-x-ray lasing with highly charged ions.Scientific reports · 2020Article
- Exploring the multiparameter nature of EUV-visible wave mixing at the FERMI FEL.Structural dynamics (Melville, N.Y.) · 2019Article
- Ultrafast dynamics of spin and orbital correlations in quantum materials: an energy- and momentum-resolved perspective.Philosophical transactions. Series A, Mathematical, physical, and engineering sciences · 2019Article
- Stimulated X-Ray Emission Spectroscopy in Transition Metal Complexes.Physical review letters · 2018Article
- In situ single-shot diffractive fluence mapping for X-ray free-electron laser pulses.Nature communications · 2018Article
- Perspective: Opportunities for ultrafast science at SwissFEL.Structural dynamics (Melville, N.Y.) · 2017Article
- EUV stimulated emission from MgO pumped by FEL pulses.Structural dynamics (Melville, N.Y.) · 2017Article
- Establishing nonlinearity thresholds with ultraintense X-ray pulses.Scientific reports · 2016Article
- Coherent control of long-range photoinduced electron transfer by stimulated X-ray Raman processes.Proceedings of the National Academy of Sciences of the United States of America · 2016Article
- Study of double core hole excitations in molecules by X-ray double-quantum-coherence signals: a multi-configuration simulation.Chemical science · 2016Article
- A beam branching method for timing and spectral characterization of hard X-ray free-electron lasers.Structural dynamics (Melville, N.Y.) · 2016Article
- Atomic inner-shell laser at 1.5-ångström wavelength pumped by an X-ray free-electron laser.Nature · 2015Article
- Article
- Monitoring Long-Range Electron Transfer Pathways in Proteins by Stimulated Attosecond Broadband X-ray Raman Spectroscopy.The journal of physical chemistry letters · 2014Article
Corrections and comments
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Authors and funding
8 authors at 3 institutions in 1 country.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Resonant inelastic X-ray scattering and X-ray emission spectroscopy can be used to probe the energy and dispersion of the elementary low-energy excitations that govern functionality in matter: vibronic, charge, spin and orbital excitations. A key drawback of resonant inelastic X-ray scattering has been the need for high photon densities to compensate for fluorescence yields of less than a per cent for soft X-rays. Sample damage from the dominant non-radiative decays thus limits the materials to which such techniques can be applied and the spectral resolution that can be obtained. A means of improving the yield is therefore highly desirable. Here we demonstrate stimulated X-ray emission for crystalline silicon at photon densities that are easily achievable with free-electron lasers. The stimulated radiative decay of core excited species at the expense of non-radiative processes reduces sample damage and permits narrow-bandwidth detection in the directed beam of stimulated radiation. We deduce how stimulated X-ray emission can be enhanced by several orders of magnitude to provide, with high yield and reduced sample damage, a superior probe for low-energy excitations and their dispersion in matter. This is the first step to bringing nonlinear X-ray physics in the condensed phase from theory to application.
Identifiers
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.