ArticleThe journal of physical chemistry letters2013
Quantum Beats and Coherence Decay in Degenerate States Split by Solvation.
Article in The journal of physical chemistry letters, 2013. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- A polarization scheme that resolves cross-peaks with transient absorption and eliminates diagonal peaks in 2D spectroscopy.Proceedings of the National Academy of Sciences of the United States of America · 2022Article
- Dynamics of Dicyanamide in Ionic Liquids is Dominated by Local Interactions.The journal of physical chemistry. B · 2019Article
- Hydration and vibrational dynamics of betaine (N,N,N-trimethylglycine).The Journal of chemical physics · 2015Article
- Kinetics of exchange between zero-, one-, and two-hydrogen-bonded states of methyl and ethyl acetate in methanol.The journal of physical chemistry. B · 2015Article
- Non-linear infrared spectroscopy of the water bending mode: direct experimental evidence of hydration shell reorganization?Physical chemistry chemical physics : PCCP · 2014Article
- Quantum process tomography quantifies coherence transfer dynamics in vibrational exciton.The journal of physical chemistry. B · 2013Article
- Vibrational dynamics of a non-degenerate ultrafast rotor: the (C12,C13)-oxalate ion.The Journal of chemical physics · 2013Article
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Authors and funding
5 authors.
Funding
Abstract
Coherent dynamics of degenerate quantum states symmetry-broken on the femtosecond timescale is found to exhibit the phenomenon of quantum beats. Frequency-resolved and polarization-selective heterodyned transient grating spectroscopy enabled us to retrieve the oscillation pattern characteristic of the beating in systems undergoing ultrafast dynamical processes. This methodology applies to the general phenomena of coherence dynamics which is important in any ultrafast multidimensional spectroscopy. A particular application to the vibrational spectroscopy of coherence in the degenerate normal modes of the tricyanomethanide anion solvated in water is explored in this study. The relaxation of the cross-polarization transient grating anisotropy is shown to reflect the loss of the vibrational coherence, which is caused by ultrafast dynamics of the water solvation shell.
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