ArticlePhysical chemistry chemical physics : PCCP2013
Broadband infrared and Raman probes of excited-state vibrational molecular dynamics: simulation protocols based on loop diagrams.
Article in Physical chemistry chemical physics : PCCP, 2013. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Capturing photochemical and photophysical transformations in iron complexes with ultrafast X-ray spectroscopy and scattering.Chemical science · 2021Review
- Nonadiabatic effects in electronic and nuclear dynamics.Structural dynamics (Melville, N.Y.) · 2017Review
- Monitoring conical intersections in the ring opening of furan by attosecond stimulated X-ray Raman spectroscopy.Structural dynamics (Melville, N.Y.) · 2016Article
- Stochastic Liouville equations for femtosecond stimulated Raman spectroscopy.The Journal of chemical physics · 2015Article
- Femtosecond stimulated Raman spectroscopy of the cyclobutane thymine dimer repair mechanism: a computational study.Journal of the American Chemical Society · 2014Article
- Stimulated Raman Spectroscopy with Entangled Light: Enhanced Resolution and Pathway Selection.The journal of physical chemistry letters · 2014Article
- Probing the Conical Intersection Dynamics of the RNA Base Uracil by UV-Pump Stimulated-Raman-Probe Signals; Ab Initio Simulations.Journal of chemical theory and computation · 2014Article
- Time-resolved broadband Raman spectroscopies: a unified six-wave-mixing representation.The Journal of chemical physics · 2013Article
- Monitoring Non-Adiabatic Dynamics of the RNA Base Uracil by UV-Pump-IR-Probe Spectroscopy.The journal of physical chemistry letters · 2013Article
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Authors and funding
3 authors.
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Abstract
Vibrational motions in electronically excited states can be observed either by time and frequency resolved infrared absorption or by off resonant stimulated Raman techniques. Multipoint correlation function expressions are derived for both signals. Three representations which suggest different simulation protocols for the signals are developed. These are based on the forward and the backward propagation of the wavefunction, sum over state expansion using an effective vibrational Hamiltonian or a semiclassical treatment of a bath. We show that the effective temporal (Δt) and spectral (Δω) resolution of the techniques is not controlled solely by experimental knobs but also depends on the system dynamics being probed. The Fourier uncertainty ΔωΔt > 1 is never violated.
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