ArticleProceedings of the National Academy of Sciences of the United States of America2013
Possible relation of water structural relaxation to water anomalies.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2013. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 14 papers.
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Who cites it
14 citing papers in PubMed.
- From Upconversion Nanoparticles to Proteins: Probing Hydration-Water Density Fluctuations by Luminescence Thermometry.Accounts of chemical research · 2026Article
- Nature of boson peak and associated heat capacity anomaly caused by structural and proton disorder in IScientific reports · 2025Article
- Deciphering Density Fluctuations in the Hydration Water of Brownian Nanoparticles via Upconversion Thermometry.The journal of physical chemistry letters · 2024Article
- The Hydrophobic Effect Studied by Using Interacting Colloidal Suspensions.International journal of molecular sciences · 2023Article
- A new one-site coarse-grained model for water: Bottom-up many-body projected water (BUMPer). II. Temperature transferability and structural properties at low temperature.The Journal of chemical physics · 2021Article
- Some Aspects of the Liquid Water Thermodynamic Behavior: From The Stable to the Deep Supercooled Regime.International journal of molecular sciences · 2020Article
- Specific Heat and Transport Functions ofWater.International journal of molecular sciences · 2020Article
- The Proton Density of States in Confined Water (HInternational journal of molecular sciences · 2019Article
- Nanoscale transient gratings excited and probed by extreme ultraviolet femtosecond pulses.Science advances · 2019Article
- Water Is a Cagey Liquid.Journal of the American Chemical Society · 2018Article
- How Water's Properties Are Encoded in Its Molecular Structure and Energies.Chemical reviews · 2017Article
- The hydrogen-bond network of water supports propagating optical phonon-like modes.Nature communications · 2016Article
- High accuracy thermal conductivity measurement of aqueous cryoprotective agents and semi-rigid biological tissues using a microfabricated thermal sensor.Scientific reports · 2015Article
- Supercooled water escaping from metastability.Scientific reports · 2014Article
Corrections and comments
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Authors and funding
3 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The anomalous behavior of thermodynamic response functions is an unsolved problem in the physics of water. The mechanism that gives rise to the dramatic indefinite increase at low temperature in the heat capacity, the compressibility, and the coefficient of thermal expansion, is unknown. We explore this problem by analyzing both new and existing experimental data on the power spectrum S(Q, ω) of bulk and confined water at ambient pressure. When decreasing the temperature, we find that the liquid undergoes a structural transformation coinciding with the onset of an extended hydrogen bond network. This network onset seems to give rise to the marked viscoelastic behavior, consistent with the interesting possibility that the sound velocity and response functions of water depend upon both the frequency and wave vector.
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