ArticleSoft matter2012
Generalized localization model of relaxation in glass-forming liquids.
Article in Soft matter, 2012. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 21 papers.
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Who cites it
21 citing papers in PubMed.
- Segmental Interaction Energy Controls a Wide Range of Material Behavior.Macromolecules · 2026Article
- A molecular dynamics study of the structure and dynamics of screened polyelectrolyte complex materials.Soft matter · 2026Article
- The role of excitations in supercooled liquids: Density, geometry, and relaxation dynamics.Proceedings of the National Academy of Sciences of the United States of America · 2025Article
- Do Specific Ion Effects on Collective Relaxation Arise from Perturbation of Hydrogen-Bonding Network Structure?The journal of physical chemistry. B · 2024Article
- Influence of swelling on the elasticity of polymer networks cross-linked in the melt state: Test of the localization model of rubber elasticity.The Journal of chemical physics · 2024Article
- Local vs. cooperative: Unraveling glass transition mechanisms with SEER.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- Comparison of Friction Parametrization from Dynamics and Material Properties for a Coarse-Grained Polymer Melt.The journal of physical chemistry. B · 2023Article
- Temperature Dependence of Structural Relaxation in Glass-Forming Liquids and Polymers.Entropy (Basel, Switzerland) · 2022Review
- Localization model description of the interfacial dynamics of crystalline Cu andThe European physical journal. E, Soft matter · 2021Article
- Dynamically consistent coarse-grain simulation model of chemically specific polymer melts via friction parameterization.The Journal of chemical physics · 2021Article
- Systematic Coarse-graining of Epoxy Resins with Machine Learning-Informed Energy Renormalization.npj computational materials · 2021Article
- Glass transition temperature from the chemical structure of conjugated polymers.Nature communications · 2020Article
- Vibrational scaling of the heterogeneous dynamics detected by mutual information.The European physical journal. E, Soft matter · 2019Article
- Fast Vibrational Modes and Slow Heterogeneous Dynamics in Polymers and Viscous Liquids.International journal of molecular sciences · 2019Review
- Universal behavior of the apparent fragility in ultraslow glass forming systems.Scientific reports · 2019Article
- Energy renormalization for coarse-graining polymers having different segmental structures.Science advances · 2019Article
- Tuning the Relaxation of Nanopatterned Polymer Films with Polymer-Grafted Nanoparticles: Observation of Entropy-Enthalpy Compensation.Nano letters · 2018Article
- Energy Renormalization for Coarse-Graining the Dynamics of a Model Glass-Forming Liquid.The journal of physical chemistry. B · 2018Article
- Sucrose diffusion in aqueous solution.Physical chemistry chemical physics : PCCP · 2016Article
- Quantitative relations between cooperative motion, emergent elasticity, and free volume in model glass-forming polymer materials.Proceedings of the National Academy of Sciences of the United States of America · 2015Article
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Authors and funding
5 authors.
Funding
Abstract
Glassy solidification is characterized by two essential phenomena: localization of the solidifying material's constituent particles and a precipitous increase in its structural relaxation time τ. Determining how these two phenomena relate is key to understanding glass formation. Leporini and coworkers have recently argued that τ universally depends on a localization length-scale <u(2)> (the Debye-Waller factor) in a way that depends only upon the value of <u(2)> at the glass transition. Here we find that this 'universal' model does not accurately describe τ in several simulated and experimental glass-forming materials. We develop a new localization model of solidification, building upon the classical Hall-Wolynes and free volume models of glass formation, that accurately relates τ to <u(2)> in all systems considered. This new relationship is based on a consideration of the the anisotropic nature of particle localization. The model also indicates the presence of a particle delocalization transition at high temperatures associated with the onset of glass formation.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.