ArticleScientific reports2012
Interplay of the glass transition and the liquid-liquid phase transition in water.
Article in Scientific reports, 2012. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 25 papers.
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Who cites it
25 citing papers in PubMed.
- Characterizing the Peierls-Like Distortion and Phase Behavior in Amorphous Ge-Sb Mixtures Using a Machine-Learned Potential.The journal of physical chemistry. C, Nanomaterials and interfaces · 2026Article
- Computational investigation of water glasses using machine-learning potentials.Proceedings of the National Academy of Sciences of the United States of America · 2025Article
- Multicomponent dynamics in amorphous ice studied using X-ray photon correlation spectroscopy at elevated pressure and cryogenic temperatures.Communications chemistry · 2025Article
- Nuclear quantum effects on glassy water under pressure: Vitrification and pressure-induced transformations.The Journal of chemical physics · 2024Article
- Potential energy landscape formalism for quantum molecular liquids.Communications chemistry · 2024Article
- Solvent constraints for biopolymer folding and evolution in extraterrestrial environments.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- A continuum of amorphous ices between low-density and high-density amorphous ice.Communications chemistry · 2024Article
- The Importance of Nuclear Quantum Effects on the Thermodynamic and Structural Properties of Low-Density Amorphous Ice: A Comparison with Hexagonal Ice.The journal of physical chemistry. B · 2023Article
- Nuclear quantum effects on the dynamics and glass behavior of a monatomic liquid with two liquid states.The Journal of chemical physics · 2022Article
- Evidence of a liquid-liquid phase transition in H[Formula: see text]O and D[Formula: see text]O from path-integral molecular dynamics simulations.Scientific reports · 2022Article
- Direct observation of reversible liquid-liquid transition in a trehalose aqueous solution.Proceedings of the National Academy of Sciences of the United States of America · 2022Article
- Advances in the study of supercooled water.The European physical journal. E, Soft matter · 2021Review
- Glasses denser than the supercooled liquid.Proceedings of the National Academy of Sciences of the United States of America · 2021Article
- Manifestations of metastable criticality in the long-range structure of model water glasses.Nature communications · 2021Article
- Nuclear quantum effects on the thermodynamic, structural, and dynamical properties of water.Physical chemistry chemical physics : PCCP · 2021Article
- X-ray studies of the transformation from high- to low-density amorphous water.Philosophical transactions. Series A, Mathematical, physical, and engineering sciences · 2019Article
- Calorimetric study of water's two glass transitions in the presence of LiCl.Physical chemistry chemical physics : PCCP · 2018Article
- Experimental evidence of low-density liquid water upon rapid decompression.Proceedings of the National Academy of Sciences of the United States of America · 2018Article
- Supercooled and glassy water: Metastable liquid(s), amorphous solid(s), and a no-man's land.Proceedings of the National Academy of Sciences of the United States of America · 2017Article
- Water: A Tale of Two Liquids.Chemical reviews · 2016Article
Corrections and comments
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Authors and funding
4 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Water has multiple glassy states, often called amorphous ices. Low-density (LDA) and high-density (HDA) amorphous ice are separated by a dramatic, first-order like phase transition. It has been argued that the LDA-HDA transformation connects to a first-order liquid-liquid phase transition (LLPT) above the glass transition temperature T(g). Direct experimental evidence of the LLPT is challenging to obtain, since the LLPT occurs at conditions where water rapidly crystallizes. In this work, we explore the implications of a LLPT on the pressure dependence of T(g)(P) for LDA and HDA by performing computer simulations of two water models - one with a LLPT, and one without. In the absence of a LLPT, T(g)(P) for all glasses nearly coincide. When there is a LLPT, different glasses exhibit dramatically different T(g)(P) which are directly linked with the LLPT. Available experimental data for T(g)(P) are only consistent with the scenario including a LLPT.
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Registered trials
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