ReviewCellular & molecular biology letters2011
Generalized stern models of the electric double layer considering the spatial variation of permittvity and finite size of ions in saturation regime.
Review in Cellular & molecular biology letters, 2011. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 11 papers.
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Who cites it
11 citing papers in PubMed.
- Tutorial on computing nonadiabatic proton-coupled electron transfer rate constants.The Journal of chemical physics · 2025Article
- Elucidation of the pH-Dependent Electric Double Layer Structure at the Positively Charged Amorphous Alumina/Water Interface Using Heterodyne-Detected Vibrational Sum-Frequency Generation.Journal of the American Chemical Society · 2025Article
- Elucidation of the pH-Dependent Electric Double Layer Structure at the Silica/Water Interface Using Heterodyne-Detected Vibrational Sum Frequency Generation Spectroscopy.Journal of the American Chemical Society · 2023Article
- Effects of Cold Atmospheric Plasma Pre-Treatment of Titanium on the Biological Activity of Primary Human Gingival Fibroblasts.Biomedicines · 2023Article
- Molecular Mean-Field Theory of Ionic Solutions: A Poisson-Nernst-Planck-Bikerman Model.Entropy (Basel, Switzerland) · 2020Review
- Resolving Anomalies in Predicting Electrokinetic Energy Conversion Efficiencies of Nanofluidic Devices.Scientific reports · 2015Article
- Membrane potential generated by ion adsorption.Membranes · 2014Article
- Interaction between dipolar lipid headgroups and charged nanoparticles mediated by water dipoles and ions.International journal of molecular sciences · 2013Article
- Spatial variation of permittivity of an electrolyte solution in contact with a charged metal surface: a mini review.Computer methods in biomechanics and biomedical engineering · 2013Review
- Stability of membranous nanostructures: a possible key mechanism in cancer progression.International journal of nanomedicine · 2012Article
- Adhesion of osteoblasts to a nanorough titanium implant surface.International journal of nanomedicine · 2011Article
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Authors and funding
3 authors.
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Abstract
The interaction between a charged metal implant surface and a surrounding body fluid (electrolyte solution) leads to ion redistribution and thus to formation of an electrical double layer (EDL). The physical properties of the EDL contribute essentially to the formation of the complex implant-biosystem interface. Study of the EDL began in 1879 by Hermann von Helmholtz and still today remains a scientific challenge. The present mini review is focused on introducing the generalized Stern theory of an EDL, which takes into account the orientational ordering of water molecules. To ascertain the plausibility of the generalized Stern models described, we follow the classical model of Stern and introduce two Langevin models for spatial variation of the relative permittivity for point-like and finite sized ions. We attempt to uncover the subtle interplay between water ordering and finite sized ions and their impact on the electric potential near the charged implant surface. Two complementary effects appear to account for the spatial dependency of the relative permittivity near the charged implant surface - the dipole moment vectors of water molecules are predominantly oriented towards the surface and water molecules are depleted due to the accumulation of counterions. At the end the expressions for relative permittivity in both Langevin models were generalized by also taking into account the cavity and reaction field.
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