ArticleThe Journal of chemical physics2010
Increasing correlation length in bulk supercooled H2O, D2O, and NaCl solution determined from small angle x-ray scattering.
Article in The Journal of chemical physics, 2010. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 15 papers.
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Who cites it
15 citing papers in PubMed.
- Supercritical density fluctuations and structural heterogeneity in supercooled water-glycerol microdroplets.Nature communications · 2024Article
- Enhancement and maximum in the isobaric specific-heat capacity measurements of deeply supercooled water using ultrafast calorimetry.Proceedings of the National Academy of Sciences of the United States of America · 2021Article
- A new one-site coarse-grained model for water: Bottom-up many-body projected water (BUMPer). II. Temperature transferability and structural properties at low temperature.The Journal of chemical physics · 2021Article
- The nano-structural inhomogeneity of dynamic hydrogen bond network of TIP4P/2005 water.Scientific reports · 2020Article
- Coherent X-rays reveal the influence of cage effects on ultrafast water dynamics.Nature communications · 2018Article
- Towards ultrafast dynamics with split-pulse X-ray photon correlation spectroscopy at free electron laser sources.Nature communications · 2018Article
- Small-angle scattering and morphologies of ultra-flexible microemulsions.Journal of applied crystallography · 2016Article
- Water: A Tale of Two Liquids.Chemical reviews · 2016Article
- The structural origin of anomalous properties of liquid water.Nature communications · 2015Review
- Ultrafast X-ray probing of water structure below the homogeneous ice nucleation temperature.Nature · 2014Article
- Effect of hydrophobic environments on the hypothesized liquid-liquid critical point of water.Journal of biological physics · 2012Article
- Nanoscale dynamics of phase flipping in water near its hypothesized liquid-liquid critical point.Scientific reports · 2012Article
- Structural transformation in supercooled water controls the crystallization rate of ice.Nature · 2011Article
- Increased fraction of low-density structures in aqueous solutions of fluoride.The Journal of chemical physics · 2011Article
- The structure of water in the hydration shell of cations from x-ray Raman and small angle x-ray scattering measurements.The Journal of chemical physics · 2011Article
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Authors and funding
6 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Using small angle x-ray scattering, we find that the correlation length of bulk liquid water shows a steep increase as temperature decreases at subzero temperatures (supercooling) and that it can, similar to the thermodynamic response functions, be fitted to a power law. This indicates that the anomalous properties of water are attributable to fluctuations between low- and high-density regions with rapidly growing average size upon supercooling. The substitution of H(2)O with D(2)O, as well as the addition of NaCl salt, leads to substantial changes of the power law behavior of the correlation length. Our results are consistent with the proposed existence of a liquid-liquid critical point in the deeply supercooled region but do not exclude a singularity-free model.
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